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Synthesis and Application of Catalytic Materials in Energy and Environment,...
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Synthesis and Application of Catalytic Materials in Energy and Environment, 2nd Edition

A special issue of Catalysts (ISSN 2073-4344). This special issue belongs to the section "Environmental Catalysis".

Deadline for manuscript submissions: closed (29 February 2024) | Viewed by 4889

Special Issue Editors

Dr. Ning Han

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Guest Editor
Department of Materials Engineering, KU Leuven, Kasteelpark Arenberg 44, 3001 Leuven, Belgium
Interests: oxide catalysts; electrocatalysis; environmental catalysis
Special Issues, Collections and Topics in MDPI journals
Dr. Zhijie Chen

E-Mail Website
Guest Editor
School of Civil and Environmental Engineering, University of Technology Sydney, Ultimo, NSW 2007, Australia
Interests: froth flotation; ore beneficiation; waste utilization; mineral materials; electrochemistry; environmental functional materials
Dr. Bo Jiang

E-Mail Website
Guest Editor
School of Energy and Power Engineering, Dalian University of Technology, Dalian 116024, China
Interests: hydrogen energy; heterogeneous catalysis; thermocatalysis; chemical reaction engineering
Special Issues, Collections and Topics in MDPI journals
Dr. Guoxing Chen

E-Mail Website
Guest Editor
Fraunhofer Research Institution for Materials Recycling and Resource Strategies IWKS, 63755 Alzenau, Germany
Interests: CO2 conversion; plasma catalysis; gas separation; perovskites; H2 production; oxygen transporting membranes; waste materials recycling
Special Issues, Collections and Topics in MDPI journals
Dr. Lingbao Xing

E-Mail Website
Guest Editor
School of Chemistry and Chemical Engineering, Shandong University of Technology, Zibo 255000, China
Interests: photocatalysis; supramolecular photochemistry; host-guest chemistry; light-harvesting; energy transfer

Special Issue Information

Dear Colleagues,

This issue is a continuation of the previous successful Special Issue “Synthesis and Application of Catalytic Materials in Energy and Environment”.

Catalytic materials have risen to prominence in many high-tech fields. These materials are not categorized according to their nature, bonding form, or processing methods, but rather according to the functions they may perform. The emergence of catalytic materials in the applications of Energy (energy storage, conversion, utilization) and Environment (detection, protection, rehabilitation) has received much more attention from both academic and industry scientists. Thus, it is necessary to provide a platform for the researchers and engineers for discussing the development of catalytic materials in energy and environment.

This Special Issue is devoted to ‘’Synthesis and Application of Catalytic Materials in Energy and Environment’’, including the synthesis, characterization, application, and mechanism analysis of the homogeneous and heterogeneous catalysts in energy and environment. All studies (experimental and theoretical) in the scope of this Special Issue, including original research and review articles, short communications, and perspective articles, are invited for submission.

Dr. Ning Han
Dr. Zhijie Chen
Dr. Bo Jiang
Dr. Guoxing Chen
Dr. Lingbao Xing
Guest Editors

Manuscript Submission Information

Manuscripts should be submitted online at www.mdpi.com by registering and logging in to this website. Once you are registered, click here to go to the submission form. Manuscripts can be submitted until the deadline. All submissions that pass pre-check are peer-reviewed. Accepted papers will be published continuously in the journal (as soon as accepted) and will be listed together on the special issue website. Research articles, review articles as well as short communications are invited. For planned papers, a title and short abstract (about 100 words) can be sent to the Editorial Office for announcement on this website.

Submitted manuscripts should not have been published previously, nor be under consideration for publication elsewhere (except conference proceedings papers). All manuscripts are thoroughly refereed through a single-blind peer-review process. A guide for authors and other relevant information for submission of manuscripts is available on the Instructions for Authors page. Catalysts is an international peer-reviewed open access monthly journal published by MDPI.

Please visit the Instructions for Authors page before submitting a manuscript. The Article Processing Charge (APC) for publication in this open access journal is 2700 CHF (Swiss Francs). Submitted papers should be well formatted and use good English. Authors may use MDPI's English editing service prior to publication or during author revisions.

Keywords

  • energy storage
  • energy conversion
  • energy utilization
  • environment rehabilitation
  • electrocatalysis
  • photocatalysis
  • H2 production
  • N2 fixation
  • CO2 conversion
  • homogeneous catalysis
  • heterogeneous catalysis
  • green synthesis

Published Papers (4 papers)

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Research

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12 pages, 2436 KiB  
Article
The Influence of Sulfurization and Carbonization on Mo-Based Catalysts for CH3SH Synthesis
by Hao Wang, Wenjun Zhang, Dalong Zheng, Yubei Li, Jian Fang, Min Luo, Jichang Lu and Yongming Luo
Catalysts 2024, 14(3), 190; https://doi.org/10.3390/catal14030190 - 11 Mar 2024
Viewed by 798
Abstract
Sulfur-resistant Mo-based catalysts have become promising for the one-step synthesis of methanethiol (CH3SH) from CO/H2/H2S, but the low reactant conversion and poor product selectivity have constrained its development. Herein, we synthesized K-MoS2/Al2O3 [...] Read more.
Sulfur-resistant Mo-based catalysts have become promising for the one-step synthesis of methanethiol (CH3SH) from CO/H2/H2S, but the low reactant conversion and poor product selectivity have constrained its development. Herein, we synthesized K-MoS2/Al2O3 and K-Mo2C/Al2O3 catalysts via the sulfurization and carbonization of K-Mo-based catalysts in the oxidized state, respectively. During the synthesis of CH3SH, both K-Mo2C/Al2O3 and K-MoS2/Al2O3 showed excellent catalytic performance, and the activity of the former is superior to that of the latter. The effect of different treatments on the catalytic performance of Mo-based catalysts was investigated by XRD, BET, Raman spectroscopy, H2-TPR, and reactants-TPD characterization. The results showed that the sulfide-treated sample showed stronger metal-support interactions and contributed to the formation of K2S, which exposed more active sites and stabilized the formation of C-S bonds. Carbonized samples enhanced the activation of H2, which promoted the hydrogenation of the intermediate species of carbonyl sulfide (COS) and thus improved the selectivity of CH3SH. Full article
(This article belongs to the Special Issue Synthesis and Application of Catalytic Materials in Energy and Environment, 2nd Edition)
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22 pages, 10846 KiB  
Article
Cobalt–Magnesium Oxide Catalysts for Deep Oxidation of Hydrocarbons
by Magira Zhylkybek, Bolatbek Khussain, Alexandr Sass, Ivan Torlopov, Tolkyn Baizhumanova, Svetlana Tungatarova, Alexandr Brodskiy, Galina Xanthopoulou, Kenzhegul Rakhmetova, Rabiga Sarsenova, Kaysar Kassymkan and Yermek Aubakirov
Catalysts 2024, 14(2), 136; https://doi.org/10.3390/catal14020136 - 09 Feb 2024
Viewed by 1057
Abstract
Co–Mg catalysts for methane combustion were synthesized and studied, revealing the transformation of MgCo2O4 spinel into a CoO–MgO solid solution with oxygen release from the spinel lattice as the calcination temperature increased. Repeated heat treatment of the calcined solid solution [...] Read more.
Co–Mg catalysts for methane combustion were synthesized and studied, revealing the transformation of MgCo2O4 spinel into a CoO–MgO solid solution with oxygen release from the spinel lattice as the calcination temperature increased. Repeated heat treatment of the calcined solid solution at lower temperatures led to spinel regeneration with segregation of the solid solution phase. A TPR of the samples showed the presence of two characteristic peaks, the first of which relates to the transition of Co3+Oh spinel to the Co2+Oh structure of CoO, and the second to the reduction of CoO to Co°. The second peak was observed at 540–620 °C for samples calcined at temperatures below spinel decomposition, and for high-temperature samples at 900–1100 °C. Taking into account the identity of the structure of phases obtained in both cases, the formation of not a true CoO–MgO solid solution, but rather a mixture of ordered oxides (“pseudo-solid solution”) in the low-temperature region, was postulated. A study of the activity of the samples showed the high activity of the spinel systems and a linear relationship between the activation energy of methane oxidation and the heat treatment temperature. Full article
(This article belongs to the Special Issue Synthesis and Application of Catalytic Materials in Energy and Environment, 2nd Edition)
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Review

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21 pages, 5049 KiB  
Review
Advances and Challenges in Oxygen Carriers for Chemical Looping Partial Oxidation of Methane
by Jinnan Zhang, Yuxuan Cui, Wang Si-ma, Yanqi Zhang, Yuming Gao, Pengxuan Wang and Qian Zhang
Catalysts 2024, 14(4), 246; https://doi.org/10.3390/catal14040246 - 07 Apr 2024
Viewed by 680
Abstract
To cope with global warming and increasing carbon emissions, the chemical looping process has attracted attention due to its excellent ability to convert fossil fuel and capture CO2. In this case, chemical looping partial oxidation technology has become the focus of [...] Read more.
To cope with global warming and increasing carbon emissions, the chemical looping process has attracted attention due to its excellent ability to convert fossil fuel and capture CO2. In this case, chemical looping partial oxidation technology has become the focus of attention due to its advantages in the production of syngas and hydrogen, especially with respect to the design and selection of oxygen carriers, which directly affect the efficiency of the production of syngas and hydrogen. In particular, the conversion of methane can reach 95% in the chemical looping partial oxidation of methane, and the selectivity of syngas, in the range of 700 °C to 900 °C at atmospheric pressure, can reach 99% for twenty or more cycles. In this review, from the perspective of metal oxide selection and structure regarding the chemical looping partial oxidation process, we discuss the role of oxygen carriers in the chemical looping partial oxidation cycle, in which the specific surface area, the lattice oxygen mobility, and the thermal stability are understood as the important factors affecting reactivity. We hope to summarize the design and development of efficient oxygen carriers with high oxygen-carrying capacity and syngas selectivity, as well as contribute to the selection, design, optimization, and redox reaction mechanism of redox catalysts. Full article
(This article belongs to the Special Issue Synthesis and Application of Catalytic Materials in Energy and Environment, 2nd Edition)
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19 pages, 4502 KiB  
Review
Repurposing Mining and Metallurgical Waste as Electroactive Materials for Advanced Energy Applications: Advances and Perspectives
by Fenghui Guo, Qian Chen, Zhihao Liu, Dongle Cheng, Ning Han and Zhijie Chen
Catalysts 2023, 13(9), 1241; https://doi.org/10.3390/catal13091241 - 26 Aug 2023
Cited by 7 | Viewed by 1884
Abstract
Developing cost-effective electroactive materials for advanced energy devices is vital for the sustainable development of electrochemical energy conversion/storage systems. To reduce the fabrication cost of electroactive materials (electrocatalysts and electrodes), growing attention has been paid to low-cost precursors. Recently, mining and metallurgical waste [...] Read more.
Developing cost-effective electroactive materials for advanced energy devices is vital for the sustainable development of electrochemical energy conversion/storage systems. To reduce the fabrication cost of electroactive materials (electrocatalysts and electrodes), growing attention has been paid to low-cost precursors. Recently, mining and metallurgical waste has been used to design electroactive materials, which shows great economic and environmental benefits. Herein, current achievements in the applications of mining and metallurgical waste-derived electroactive materials in sustainable energy conversion/storage fields (batteries, supercapacitors, fuel cells, and small-molecule electro-conversion) are comprehensively analyzed. The waste-to-materials conversion methods and materials’ structure–performance relationships are emphasized. In addition, perspectives related to the further development and applications of waste-derived high-performance electroactive materials are pointed out. Full article
(This article belongs to the Special Issue Synthesis and Application of Catalytic Materials in Energy and Environment, 2nd Edition)
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