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Article

Experimental Study on Rapid Determination Method of Coal Seam Gas Content by Indirect Method

1
State Key Laboratory of the Gas Disaster Detecting, Preventing and Emergency Controlling, Chongqing 400037, China
2
China Coal Technology and Engineering Group, Chongqing Research Institute, Chongqing 400037, China
*
Author to whom correspondence should be addressed.
Processes 2023, 11(3), 925; https://doi.org/10.3390/pr11030925
Submission received: 25 February 2023 / Revised: 15 March 2023 / Accepted: 16 March 2023 / Published: 17 March 2023
(This article belongs to the Special Issue Process Safety in Coal Mining)

Abstract

:
In view of the problems of heavy work, long cycle, high cost and low efficiency in the process of indirect determination of coal seam gas content, the basic gas parameters and coal quality indexes of 24 coal samples from 5 coal mines in the Hancheng area of Shanxi Province are measured by the laboratory measurement method. The raw coal gas content–gas desorption index of drilling cuttings (WK1) relationship model is characterized by logarithmic function. Using SPSS data analysis software, a stepwise multiple linear regression method is used for statistical analysis. The results show that the factors that have a significant impact on the regression slope C in the WK1 relationship model are gas adsorption constant (a), apparent density (ARD), initial velocity of gas diffusion (Δp) and consistent coefficient (f). The factors that have a significant impact on the regression constant D are Δp and atmospheric adsorption (Q). Then, the mathematical model of rapid prediction of coal seam gas content is determined. Compared with the measured values, the average absolute error rate is 12.84%, which meets the prediction requirements and provides a simple and easy method for rapid determination of coal seam gas content in coal mines in the Hancheng area.

1. Introduction

Coal seam gas content directly affects the amount of coal seam gas and the amount of mine gas emission, which are of great significance for the correct design of mine ventilation, gas drainage and outburst risk assessment [1,2,3,4]. Coal seam gas content is an important parameter to characterize the occurrence of coal seam gas. Accurate prediction of coal seam gas content plays a vital role in the prevention and control of coal mine gas disasters. The determination method of coal seam gas content is divided into the direct method and indirect method. The direct method [5,6,7] is to measure the amount of desorbable gas and normal pressure gas in the underground field and laboratory and then calculate the gas loss in the sampling process. The sum of the three parts is the gas content of the coal seam. The indirect method [8,9,10] is to measure the basic gas parameters such as gas adsorption constant, industrial analysis, density and porosity in the laboratory. Combined with the measured coal seam gas pressure in the underground field, the adsorbed gas amount and free gas amount of coal are calculated by the Langmuir equation. The sum of the two parts is the coal seam gas content. Because there are many factors affecting the gas content of coal seams [1,11,12,13,14,15], and the gas occurrence has the characteristics of complexity, nonlinearity, dynamics and random uncertainty, it is difficult to accurately determine the gas content of a coal seam. In recent years, for the prediction of coal seam gas content, Zhang et al. [16] used the method of multiple linear regression analysis. Chen et al. [17,18,19] adopted the grey theory method. Zhang et al. [20,21] used the neural network analysis method. Wang et al. [22,23] used a machine learning algorithm. They studied different mathematical models for predicting coal seam gas content. The prediction model mainly focuses on the relationship between the influencing factors such as coal seam depth, coal seam thickness, floor elevation, fault distance, coal rock dip angle and coal seam gas content. These scholars are using direct methods to predict coal seam gas content. However, there are few studies on predicting coal seam gas content by indirect methods in a laboratory. Li [24] used the drilling cuttings gas desorption index method to predict coal seam gas content. Through the study, the exponential mathematical model for predicting coal seam gas content was obtained, which avoided the determination of coal seam gas pressure. However, the regression coefficient of the exponential mathematical model is not accurately determined. Compared with the direct method, the gas basic parameters measured by the indirect method are all measured values, and the gas pressure of the coal seam is also measured. There are fewer influencing factors in the measurement process, the measurement error is small, and the measurement data is relatively reliable. However, the disadvantage of using an indirect method to measure coal seam gas content is that it is necessary to measure coal seam gas pressure underground. This is relatively heavy work, and the measurement period is long (about one month). Especially in the gently inclined coal seam or the coal seam with poor surrounding rock density, it is difficult to measure the gas pressure of the coal seam. In short, it is common that the results of a direct method are low, while the results of indirect methods in many mines are close to reality [25]. To solve the problem of accurate determination of coal seam gas pressure in the indirect determination of coal seam gas content, 24 coal samples from 5 coal mines in the Hancheng area of Shanxi Province are selected. The relationship model between gas basic parameters, coal quality index, drilling cuttings gas desorption index and gas pressure of these coal samples was measured in the laboratory. The SPSS data analysis software was used, and the stepwise multiple linear regression analysis method was used. A mathematical model for predicting the gas content of coal seams in the Hancheng area unrelated to gas pressure was established. This method can quickly and accurately determine the gas content of the coal seam in this area, and provide technical guidance and reference for mine gas disaster prevention, coal and tile outburst prediction, gas emission prediction and so on.

2. Indirect Method to Determine the Coal Seam Gas Content

2.1. Coal Seam Gas Content Calculation

The most commonly used indirect determination method of coal seam gas content at home and abroad is to calculate the coal seam gas content according to the known coal seam gas pressure and the gas adsorption constant value of coal measured in the laboratory [26]. The calculation formula is:
W = a b p 100 A a d M a d 100 1 + b p 1 + 0.31 M a d + 10 k p A R D
where W is the raw coal gas content, m3/t. a is gas adsorption constant, cm3/g. b is the gas adsorption constant, MPa−1. p is coal seam gas pressure, MPa. Aad is the ash content of coal, %. Mad is the moisture of coal, %. k is the porosity of coal, %. ARD is the apparent density of coal, t/m3.

2.2. Coal Sample Taking and Test

Four and five coal samples are taken from different sampling sites of 3# coal seam and 5# coal seam, respectively, in the Xiangshan Coal Mine in the Hancheng area of Shanxi Province. Two and three coal samples are taken from 2# coal seam and 3# coal seam, respectively, in the Xiayukou Coal Mine. Three and two coal samples are taken from 3# coal seam and 5# coal seam, respectively, in the Xinglong Coal Mine. Three coal samples are taken from 3# coal seam in the Sangbei Coal Mine. Two coal samples are taken from 3# coal seam in the Sangshuping Coal Mine. A total of 24 coal samples are taken. According to the GB/T482–2008 ‘coal seam coal sample taking method’, GB/T474–2008 ‘coal sample preparation method’, GB/T477–2008 ‘coal sample screening test method’ and other national standards, about 5 kg mixed coal samples are taken from freshly exposed coal seams, indicating the sampling location, and the packaging is strictly sent to the laboratory for drying, crushing and screening, and coal samples of different particle sizes are prepared for inspection, according to the MT/T752–1997 ‘Determination method of methane adsorption in coal’, GB/T212–2008 ‘Industrial analysis method of coal’, GB/T 217–2008 ‘Truth relative density determination method of coal’, GB/T6949–2008 ‘Apparent relative density determination method of coal’, AQ1080–2009 ‘Determination method of initial velocity index (Δp) of gas emission in coal’, GB/T23561.12–2010 ‘Determination method of firmness coefficient of coal’ and other coal industry standards and national standards. The HCA-type high-pressure capacity method gas adsorption device, industrial analysis tester, density tester, gas emission initial velocity tester, WTC gas outburst parameter tester and other instruments and equipment are used. In the laboratory, the moisture Mad, ash Aad, volatile Vdaf, true density TRD, apparent density ARD, porosity k, atmospheric adsorption Q and gas adsorption constant a and b of 24 coal samples from 5 coal mines in the Hancheng area are measured. The results of gas basic parameters of 24 coal samples are summarized.
The variation ranges of each parameter of 24 coal samples measured in Table 1 are as follows: Mad is 0.54~1.59%, Aad is 4.30~26.87%, Vdaf is 13.10~18.61%, TRD is 1.32~1.57 g·cm−3, ARD is 1.29~1.51 g·cm−3, k is 2.05~5.84%, Q is 2.1624~3.8969 cm3·g−1, a is 17.0599~26.6249 cm3·g−1, and b is 0.8217~1.7279 MPa−1. From the distribution characteristics of the measured data, the selected coal samples are universal and extensive.

3. K1p Relation Model

The drilling cuttings gas desorption index K1 characterizes the characteristic parameters of the coal gas desorption speed. It reflects the coal seam gas content and the size of the initial pressure relief gas desorption rate. Scholars at home and abroad have carried out extensive and in-depth research on the law of gas desorption from drilling cuttings in the laboratory [27,28]. They mainly studied the influence of mathematical fitting of gas desorption law and gas pressure on the gas desorption index of drilling cuttings. The research results show that the gas desorption law of drilling cuttings is the law of gas desorption amount of drilling cuttings changing with time. It can not only reflect the gas adsorption pressure and desorption gas content in coal but also reflect the damage degree of coal; that is, it can be used for outburst prediction. It is also used to determine the gas pressure and tile content of a coal seam. According to Zhao’s research results [29], there is a power function relationship between the gas desorption index of drilling cuttings and the gas pressure of adsorption equilibrium:
K 1 = m p n
where K1 is the gas desorption index of drilling cuttings, mL·g−1·min−0.5. p is the adsorption equilibrium gas pressure, MPa. m and n are undetermined constants, 0 < n < 1.
The instrument used to determine K1 in the underground field and laboratory is a WTC gas outburst parameter instrument. The underground site is measured according to the AQ/T 1065–2008 drilling cuttings gas desorption index determination method. The laboratory determination of the K1p relationship model test process is based on the test method adopted by Lei [30]. According to Equation (2), the key to determine the gas desorption index of drilling cuttings is to determine the undetermined constants m and n. The essence of laboratory determination of the K1p relationship model is to determine the undetermined constants m and n. The measured K1p relationship model results of 24 coal samples, gas basic parameters such as gas initial velocity Δp, coal firmness coefficient f and coal quality index measurement results are summarized in Table 2 below.
The variation ranges of each parameter of 24 coal samples measured in Table 2 are as follows: Δp is 7~37 mmHg, f is 0.10~0.55, K1p relationship model coefficient m is 0.217~0.9371, and index n is 0.4431~0.7740.

4. Test Result Analysis

4.1. Relationship between K and Coal Quality Index

Coal quality indexes mainly include gas emission initial velocity Δp, firmness coefficient f, volatile matter Vdaf, ash Aad, etc. They macroscopically reflect some essential characteristics related to coal and gas desorption. Among them, Δp and f are commonly used in regional outburst risk prediction. Because Δp, f, Vdaf, Aad, etc. are all coal quality indicators unrelated to gas pressure, the relationship between them and the values under certain gas pressure conditions can only be considered. In Table 2, the K1 value is calculated when the gas pressure p = 1 MPa. Through nonlinear fitting of the data in Table 1 and Table 2, the relationship between (K1)p=1 and Δp, f, Vdaf, Aad is obtained, as shown in Figure 1.
It can be seen from Figure 1a that the relationship between (K1)p=1 and Δp conforms to the power function increasing relationship. With the increase in Δp, the value of (K1)p=1 also increases correspondingly. The correlation coefficient R2 is 0.812, indicating that there is a significant correlation between K1 and Δp, and Δp significantly affects the positive (K1)p=1. It can be seen from Figure 1b that (K1)p=1 is in accordance with the logarithmic function attenuation relationship. As f increases, the value of (K1)p=1 decreases accordingly. The correlation coefficient R2 is 0.657, indicating that there is also a certain correlation between (K1)p=1 and f, and f affects negative (K1)p=1, but the significance is lower than Δp. It can be seen from Figure 1c that the distribution of 24 coal samples represented by 24 points in the figure is relatively disordered. The relationship between (K1)p=1 and Aad is an approximately logarithmic function, and the correlation coefficient R2 is only 0.129, indicating that the correlation between (K1)p=1 and Aad is not close. It can be seen from Figure 1d that 24 points are concentrated in the range of 13.10~18.61 of Vdaf, and (K1)p=1 has no correlation with Vdaf.
From the above analysis, it can be seen that under the same gas pressure condition, the value of K1 mainly depends on Δp. In theory, K1 is the same as Δp, which is an index to reflect the risk of outburst by the amount of initial gas desorption. Their fundamental difference is only the difference of adsorption gas pressure; that is, K1 index reflects the change of adsorption gas pressure more than Δp. The firmness coefficient f mainly reflects the ability of coal to resist damage. In many cases, the lower the strength of a coal seam, the greater the initial gas desorption. The regression analysis shows that under the condition of certain gas pressure, K1 decreases with the increase in f in a negative exponential law. The volatile matter Vdaf of coal reflects the metamorphic degree of coal, and the ash Aad reflects the yield of effective carbon. Both of them are not closely related to the initial gas desorption amount. In short, K1 is most affected by Δp and less affected by Vdaf and Aad. Therefore, Δp is the main influencing factor of K1, and f, Vdaf and Aad are secondary influencing factors.

4.2. The Relationship between Coal Seam Gas Content W and K1

The coal seam gas content W in Equation (1) and the drilling cuttings gas desorption index K1 in Equation (2) are directly related to the gas pressure p, and as the gas pressure increases, K1 and W increase. To find the relationship between K1 and W, gas pressure p is set to 0.1, 0.5, 1.0, 2.0, 3.0, 4.0, 5.0 MPa. Equations (1) and (2) are used to calculate 7 K1 and 7 W corresponding to 7 gas pressures, and then, the nonlinear fitting is carried out. The WK1 relationship model is obtained, and the correlation coefficient R2 is greater than 0.9900. The results are summarized in Table 2. One coal sample each (limited to the length of the article) was selected from the Xiangshan Coal Mine, Xiayukou Coal Mine, Xinglong Coal Mine, Sangbei Coal Mine and Sangshuping Coal Mine for nonlinear fitting. The fitting relationship curve is shown in Figure 2.
It can be seen from Figure 2 that there is a significant correlation between coal seam gas content W and drilling cuttings gas desorption index K1, which is characterized by logarithmic function. The WK1 relationship model can be expressed by Equation (3):
W = C ln K 1 + D
where W is the gas content of raw coal, m3/t. K1 is the gas desorption index of drilling cuttings, mL·g−1·min−0.5. C is regression slope. D is regression constant.
In the process of adsorption and desorption of coal, the change of coal seam gas content W and drilling cuttings gas desorption index K1 is caused by the change of coal seam gas pressure. This change eventually leads to the continuous change of diffusion coefficient in the process of coal desorption, which leads to the unique nonlinear relationship between W and K1. Figure 2 shows that when the gas desorption index K1 of the five coal mines is the same, the coal seam gas content W of the Xiangshan Coal Mine is the largest, and the coal seam gas content W of the Xiayukou Coal Mine is the smallest. From Table 2, the WK1 relationship model coefficient C is 4.000~7.722, and D is 9.829~17.98.

4.3. Determination of Regression Coefficient of W–K1 Relation Model

It can be seen from Equation (3) that the key is to determine the regression coefficients C and D, whether it is to determine the coal seam gas content W through the drilling cuttings gas desorption index K1 or to determine K1 through W. Although the regression coefficients C and D of the WK1 relationship model of a specific sampling site in a coal mine can be obtained through the laboratory, combined with the measured data of the underground site, this is the result based on a large amount of experimental data such as 11 gas basic parameters and coal quality indexes measured in the laboratory and the measured coal seam gas pressure and drill cuttings gas desorption index K1 in the coal mine. The determination of these parameters is heavy, long cycle, high cost and low efficiency. For the coal mines in the Hancheng area, only by finding out the universal law of the regression coefficients C and D in the WK1 relationship model and establishing a regression coefficient relationship model suitable for the area can the coal seam gas content be predicted quickly and accurately, and a simple and easy method for predicting the coal seam gas content in the Hancheng area is provided.
Taking 24 coal samples from 5 coal mines in the Hancheng area as samples, 24 regression coefficients C and 24 regression coefficients D (as shown in Table 2) obtained by the WK1 relationship model are taken as dependent variables, respectively. Mad, Aad, Vdaf, TRD, ARD, k, Q, a, b, Δp, f and another 11 gas basic parameters and coal quality indexes corresponding to coal samples are used as independent variables. The SPSS data analysis software is used. The stepwise multiple linear regression method is used for statistical analysis. According to the order of input parameters, 11 independent variables are introduced into the regression formula one by one. The regression results show that for the dependent variable C, after eliminating the seven parameters that cannot have a significant impact, the final model introduces four parameters a, ARD, Δp and f. Similarly, for the dependent variable D, after eliminating the nine parameters that cannot have a significant impact, the final model introduces two parameters such as Δp and Q. Through SPSS data analysis, the multiple linear regression model of regression coefficients C and D in the WK1 relationship model is:
C = 11.031 + 0.148 a + 0.084 Δ p 7.919 A R D + 2.263 f
D = 4.724 0.339 Δ p + 4.725 Q

4.4. Multiple Linear Regression Model Test

The prerequisites for the establishment of multiple linear regression models (4) and (5) are that there is no serious autocorrelation between series, there is no strong multicollinearity between independent variables and the residual distribution basically obeys the normal distribution. Only when these three assumptions are satisfied at the same time can it be proved that (4) and (5) have certain validity and reliability. SPSS data analysis software is used for statistical analysis of the output results (as shown in Table 3). The coefficient of determination of the regression model (4) in Table 3 is 0.833, indicating that the four independent variables a, ARD, Δp and f can explain 83.3% of the change of the dependent variable C, R2 is close to 1, and the goodness of regression fitting is better. That is to say, there is a very close linear correlation between C and a, ARD, Δp and f. The coefficient adjustment R2 of the regression model (5) is only 0.631, indicating that the two independent variables such as Δp and Q can explain 63.1% of the change in the dependent variable D, and there is a certain linear correlation between D and Δp and Q.
Regression model (4) significance level (t statistics corresponding probability value) Sig = 0.038 < 0.05. The probability that 11 independent variables cannot have a significant impact on the dependent variable C is 0. Rejecting the null hypothesis, there are at least four independent variables, a, ARD, Δp and f, that have a significant impact on C in the 11 independent variables. Among them, a, Δp and f significantly affect positive C, and ARD significantly affects negative C. The significance level of regression model (5) (the probability value corresponding to t statistics) Sig = 0.001 < 0.05, indicating that there are at least two independent variables, Δp and Q, that have a significant impact on D, where Δp significantly affects negative D and Q significantly affects positive D.
Regression models (4) and (5) Durbin-Wastson in Table 3. are 2.082 and 1.377, respectively, which are close to 2. In statistics, when the Durbin-Wastson value is significantly close to 0 or 4, the sequences are not independent of each other, and there is a serious autocorrelation. Therefore, it can be considered that the series in regression models (4) and (5) are independent of each other and there is no serious autocorrelation.
In statistics, it is generally believed that there is no strong multicollinearity between independent variables when the variance inflation factor VIF is less than 5. The output result of statistical analysis using SPSS data analysis software is that the variance expansion factor VIF of the four independent variables of a, ARD, Δp and f in the regression model (4) is 1.761, 1.771, 3.262, and 3.133, respectively, all less than 5. The variance expansion factor VIF of the two independent variables, such as Δp and Q, are 1.488 and 1.488, respectively, which are also less than 5. It shows that there is no strong multicollinearity between a, ARD, Δp and f, between Δp and Q; that is, there is no strong correlation.
From the standard PP diagram and scatter diagram of the regression standardized residuals of the dependent variables C and D in Figure 3 and Figure 4, it can be seen that the standardized residuals are basically distributed around the asymptote, the scatters are basically linear, and the data and models are basically matched. The distribution of sample points is scattered and irregular, the residuals are random, and there is no heteroscedasticity. This shows that the residual basically obeys the normal distribution.
The main factors that significantly affect the regression coefficient C are a, ARD, Δp and f, and the main factors that significantly affect the regression coefficient D are Δp and Q. There is no serious autocorrelation between the tested series, and there is no strong multicollinearity between the independent variables. The residual distribution is basically normal distribution. Therefore, the C and D regression models (4) and (5) established by SPSS data analysis software have certain validity and reliability.

5. Mathematical Model Prediction Correction of Coal Seam Gas Content

Through the above research and analysis, the regression models (4) and (5) of regression coefficients C and D are established. Substituting (4) and (5) into Equation (3), the mathematical model (6) for predicting coal seam gas content in coal mines in the Hancheng area is finally obtained:
W = ( 11.031 + 0.148 a + 0.084 Δ p 7.919 A R D + 2.263 f ) ln K 1 + ( 4.724 0.339 Δ p + 4.725 Q )
where W′ is the predicted value of coal gas content, m3/t.
Three coal samples are taken from the Xiangshan Coal Mine, Xiayukou Coal Mine and Sangbei Coal Mine in the Hancheng area. Eleven gas basic parameters and coal quality indexes of Mad, Aad, Vdaf, TRD, ARD, F, Q, a, b, Δp, f, etc. of three coal samples are measured in the laboratory. At the same time, the K1p relationship model of three coal samples is measured by a WTC gas outburst parameter instrument [31]. The gas content of the coal seam is predicted by mathematical model (6). The gas pressure p is set as 0.5, 1.0, 2.0, 3.0, 4.0 and 5.0 MPa, respectively. The predicted value W′ of the mathematical model of coal seam gas content is compared with the measured value W (as shown in Table 4).
It can be seen from Table 4 that when the gas pressure is 0.5 MPa, 1.0 MPa, 2.0 MPa, 3.0 MPa, 4.0 MPa and 5.0 MPa, the variation range of the predicted value W′ of the mathematical model of coal seam gas content and the measured value W is 3.7021~13.0581 m3/t. The predicted value W′ and the measured value W increase with the increase in gas pressure. When the gas pressure is in the range of 0.5~5.0 MPa, the maximum deviation between the predicted value W′ and the measured value W is −2.3189 m3/t when the gas pressure is 4.0 MPa in the Xiayukou Coal Mine. The minimum deviation is 0.0711 m3/t corresponding to the gas pressure of 0.5 MPa in the Xiangshan Coal Mine. The average deviation is −1.2178 m3/t. The maximum error rate is −25.71%. The minimum error rate is 1.31%. The average error rate is −12.84%.
In Figure 5, the trend of the predicted value W′ of the mathematical model of coal seam gas content in the three coal mines is generally consistent with the measured value W, which conforms to the characteristics of logarithmic function. The predicted value W′ of the Xiangshan Coal Mine is very close to the measured value W, and the change trend of the Xiayukou Coal Mine deviates far. In the low-pressure state, the coincidence degree is high, close to coincidence, and the average absolute error rate is 12.84%, which can meet the prediction requirements. It can be seen that the mathematical model of multiple linear regression has high reliability in predicting coal seam gas content in the Hancheng area. Because the average deviation is −1.2178 m3/t, the predicted value W′ is generally lower than the measured value W. Therefore, Equation (6) is modified by the average deviation of −1.2178 m3/t. The modified mathematical model is:
W = ( 11.031 + 0.148 a + 0.084 Δ p 7.919 A R D + 2.263 f ) ln K 1 + ( 4.724 0.339 Δ p + 4.725 Q ) + 1.2178

6. Conclusions

(1)
Through the experimental study and analysis of coal samples in the Hancheng area of Shanxi, it is found that W and K1 have a significant correlation. SPSS data analysis software is used for statistical analysis, and the main influencing factors of the regression coefficient C of the WK1 relationship model are a, ARD, Δp and f. Among them, a, Δp and f significantly affect positive C, and ARD significantly affects negative C. The main factors of regression coefficient D are Δp and Q, where Δp significantly affects negative D and Q significantly affects positive D. After testing, the multiple linear regression model has certain validity and reliability.
(2)
When the gas pressure is 0.5, 1.0, 2.0, 3.0, 4.0 and 5.0 MPa, the maximum deviation between the predicted value W′ of the mathematical model of coal seam gas content and the measured value W is −2.3189 m3/t, the minimum deviation is 0.0711 m3/t, and the average absolute error rate is 12.84%. It can meet the prediction requirements.
(3)
The mathematical model of predicting coal seam gas content is only related to six parameters, such as a, ARD, Δp, f, Q and K1, and has nothing to do with coal seam gas pressure. It avoids the problems of heavy task, long cycle, high cost and low efficiency in measuring coal seam gas pressure in a coal mine. The prediction model can quickly and accurately determine the gas content of a coal seam and provide a simple and feasible method for predicting the gas content of coal seams in the Hancheng area.

Author Contributions

Investigation, H.L., L.D., J.C., R.L. and B.W.; methodology, H.L., L.D. and J.C.; supervision, L.D., R.L. and B.W.; writing—original draft, H.L., L.D. and J.C.; writing—review and editing, H.L., L.D., J.C. and R.L.; funding acquisition, L.D., J.C., R.L. and B.W. All authors have read and agreed to the published version of the manuscript.

Funding

This research was funded by the National Natural Science Foundation of China (No. 51974358, No. 52104239 and No. 51874348), Natural Science Foundation of Chongqing (No. CSTB2022NSCQ-MSX1080, No. CSTB2022NSCQ-MSX0379 and No. cstc2020jcyj-msxmX1052), and Chongqing Science Fund for Distinguished Young Scholars (No. cstc2019jcyjjqX0019).

Data Availability Statement

All data and/or models used in the study appear in the submitted article.

Acknowledgments

We also would like to thank the anonymous reviewers for their valuable comments and suggestions that led to a substantially improved manuscript.

Conflicts of Interest

The authors declare no conflict of interest.

References

  1. Dai, L.C.; Lei, H.Y.; Cheng, X.Y.; Li, R.F. Prediction of coal seam gas content based on the correlation between gas basic parameters and coal quality indexes. Front. Energy Res. 2023, 10, 1096539. [Google Scholar] [CrossRef]
  2. Wang, F.K.; Zhao, X.S.; Liang, Y.P.; Li, X.L.; Chen, Y.L. Calculation model and rapid estimation method for coal seam gas content. Processes 2018, 6, 223. [Google Scholar] [CrossRef] [Green Version]
  3. Wang, L.; Cheng, L.B.; Cheng, Y.P.; Liu, S.M.; Guo, P.K.; Jin, K.; Jiang, H.N. A new method for accurate and rapid measurement of underground coal seam gas content. J. Nat. Gas Sci. Eng. 2015, 26, 1388–1398. [Google Scholar] [CrossRef]
  4. Chaffee, A.L.; Lay, G.; Marshall, M.; Jackson, W.R.; Fei, Y.; Verheyen, T.V.; Cassidy, P.J.; Scott, S.G. Structural characterisation of Middle Jurassic, high-volatile bituminous Walloon subgroup coals and correlation with the coal seam gas content. Fuel 2010, 89, 3241–3249. [Google Scholar] [CrossRef]
  5. Yan, G.Q.; Wang, G.; Xin, L.; Du, W.Z.; Huang, Q.M. Direct fitting measurement of gas content in coalbed and selection of reasonable sampling time. Int. J. Min. Sci. Technol. 2017, 27, 299–305. [Google Scholar] [CrossRef]
  6. Xu, H.J.; Ahmad, F.; Hu, B.L.; Sun, G.; Liu, H.H.; Ding, H.; Zhang, M.; Fang, H.H. Methodology for lost gas determination from exploratory coal cores and comparative evaluation of the accuracy of the direct method. ACS Omega 2021, 6, 19695–19704. [Google Scholar] [CrossRef]
  7. Zhou, F.B.; Kang, J.H.; Wang, Y.P.; Zhang, R. Method of underground integrated automatic and accurate determination of coalbed gas content. J. China Coal Soc. 2022, 47, 2873–2882. [Google Scholar] [CrossRef]
  8. Zhao, F.J.; Wen, Z.H.; Liu, M.J.; Wei, J.P.; Chen, M. Analysis content affected to seam gas pressure measured with indirect method. Coal Sci. Technol. 2010, 38, 52–54. [Google Scholar] [CrossRef]
  9. Hou, X.W.; Liu, S.M.; Zhu, Y.M.; Yang, Y. Evaluation of gas contents for a multi-seam deep coalbed methane reservoir and their geological controls: In situ direct method versus indirect method. Fuel 2020, 265, 116917. [Google Scholar] [CrossRef]
  10. Wang, Q.; Wang, Z.F.; Yue, J.W.; Wang, L.G.; Dong, J.X.; Tan, R.H. Experimental study on reasonable adsorption time in determination coalbed methane content. Geofluids 2022, 2022, 1–15. [Google Scholar] [CrossRef]
  11. Creedy, D.P. Methods for the evaluation of seam gas content from measurements on coal samples. Min. Sci. Technol. 1986, 3, 141–160. [Google Scholar] [CrossRef]
  12. Plaksin, M.S.; Kozyreva, E.N. Determining the Gas Content of Coal Beds. Coal Chem. 2021, 64, 144–147. [Google Scholar] [CrossRef]
  13. Malinnikova, O.N.; Ul’yanova, E.V.; Kharchenko, A.V.; Pashichev, B.N. Influence of coal microstructure on gas content of the face area. J. Min. Sci. 2020, 56, 351–358. [Google Scholar] [CrossRef]
  14. Li, D.; Peng, S.P.; Du, W.F.; Guo, Y.L. New method for predicting coal seam gas content. Energy Sources Part A 2019, 41, 1272–1284. [Google Scholar] [CrossRef]
  15. Li, C.W.; Wang, Y.L.; Wang, Q.J.; Gao, X. Experimental study on accuracy of direct gas. J. China Coal Soc. 2020, 45, 189–196. [Google Scholar]
  16. Zhang, J.F.; Xie, Y.D.; Yang, F.F.; Liu, G.L.; Zhang, J.J.; Miao, Z.Q.; Ma, D.Q. Study on prediction method of coal seam gas content based on principal component multiple regression. Int. J. Oil Gas Sci. Eng. 2020, 2, 1–7. [Google Scholar]
  17. Chen, Y.Q.; Zheng, L.J.; Huang, J.; Zou, Z.; Li, C.H. Prediction of gas emission based on grey-generalized regression neural network. IOP Conf. Ser. Earth Environ. Sci. 2020, 467, 012056. [Google Scholar] [CrossRef]
  18. Xu, G.; Wang, L.; Wang, H.T.; Wang, K.; Feng, Y.Z. Prediction method of coal seam gas content based on Grey theory and BP Neural Network. Coal Technol. 2019, 38, 82–85. [Google Scholar]
  19. Wu, X.; Yang, Z.; Wu, D.D. Advanced computational methods for mitigating shock and vibration hazards in deep mines gas outburst prediction using SVM optimized by Grey relational analysis and APSO algorithm. Shock Vib. 2021, 2021, 5551320. [Google Scholar] [CrossRef]
  20. Zhang, J.Q. Study on the gas content of coal seam based on the BP Neural Network. Procedia Eng. 2011, 26, 1554–1562. [Google Scholar]
  21. Lv, Y.N.; Tang, D.Z.; Xu, H.; Tao, S. Productivity matching and quantitative prediction of coalbed methane wells based on BP neural network. Sci. China Technol. Sci. 2011, 54, 1281–1286. [Google Scholar]
  22. Wang, L.; Li, J.H.; Zhang, W.B.; Li, Y. Research on the gas emission quantity prediction model of improved artificial bee colony algorithm and weighted least squares support vector machine (IABC-WLSSVM). Appl. Bionics Biomech. 2022, 2022, 4792988. [Google Scholar] [CrossRef] [PubMed]
  23. Guo, J.H.; Zhang, Z.S.; Guo, G.S.; Xiao, H.; Zhu, L.Q.; Zhang, C.M.; Tang, X.; Zhou, X.Q.; Zhang, Y.N.; Wang, C. Evaluation of coalbed methane content by using Kernel Extreme Learning Machine and Geophysical Logging Data. Geofluids 2022, 2022, 1–28. [Google Scholar] [CrossRef]
  24. Li, X.J. Experimental Research on the relationship between gas desorption index of drill cuttings and gas content. Saf. Coal Mines 2014, 45, 8–12. [Google Scholar]
  25. Huang, H.X.; Sun, W.; Xiong, F.Y.; Chen, L.; Li, X.; Gao, T.; Jiang, Z.X.; Ji, W.; Wu, Y.J.; Han, J. A novel method to estimate subsurface shale gas capacities. Fuel 2018, 232, 341–350. [Google Scholar] [CrossRef]
  26. Lei, H.Y.; Pang, J.L.; Chen, Y.T.; Cao, J. Experimental study on calibration of calculation formula of gas content in coal seam by indirect method. Min. Saf. Environ. Prot. 2018, 45, 37–40. [Google Scholar]
  27. Ma, S.Y. Selection of characteristic particle size of drilling cuttings based on adsorption–desorption properties: Experiment and Simulation. Adsorpt. Sci. Technol. 2022, 2022, 1–19. [Google Scholar] [CrossRef]
  28. Kong, S.L.; Cheng, L.B.; Wang, H.F.; Zhou, H.X. Determination and application on critical value of drilling cuttings gas desorption indices. Coal Sci. Technol. 2014, 42, 56–59+64. [Google Scholar]
  29. Zhao, X.S.; Dong, Y.S.; Yue, C.P. Method for determining the sensitive index of coal and gas outburst prediction and its critical value. Min. Saf. Environ. Prot. 2007, 34, 28–30+52+89. [Google Scholar]
  30. Lei, H.Y. Experimental study on rapid determination of critical value of drilling cutting gas desorption index. Coal Sci. Technol. 2019, 47, 129–134. [Google Scholar]
  31. Zhu, T.H.; Zhang, Y.Z.; Xie, A.F.; Li, W.B.; Jiang, P.F. Upgrading and optimization of gas outburst parameter measuring instrument and its on-site comparative investigation and application. Ind. Saf. Environ. Prot. 2021, 47, 48–50. [Google Scholar]
Figure 1. Relationship between (K1)p=1 and coal quality index. (a) Relationship between (K1)p=1 and Δp. (b) Relationship between (K1)p=1 and f . (c) Relationship between (K1)p=1 and Aad. (d) Relationship between (K1)p=1 and Vdaf.
Figure 1. Relationship between (K1)p=1 and coal quality index. (a) Relationship between (K1)p=1 and Δp. (b) Relationship between (K1)p=1 and f . (c) Relationship between (K1)p=1 and Aad. (d) Relationship between (K1)p=1 and Vdaf.
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Figure 2. The relationship between W and K1.
Figure 2. The relationship between W and K1.
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Figure 3. Standard PP diagram and scatter plot diagram of regression normalized residual of dependent variable C. (a) Cumulative probability of observation. (b) Regression standardized predicted value.
Figure 3. Standard PP diagram and scatter plot diagram of regression normalized residual of dependent variable C. (a) Cumulative probability of observation. (b) Regression standardized predicted value.
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Figure 4. Standard PP diagram and scatter plot diagram of regression normalized residual of dependent variable D. (a) Cumulative probability of observation. (b) Regression standardized predicted value.
Figure 4. Standard PP diagram and scatter plot diagram of regression normalized residual of dependent variable D. (a) Cumulative probability of observation. (b) Regression standardized predicted value.
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Figure 5. The predicted value W′ of the regression model under different pressures is compared with the measured value W.
Figure 5. The predicted value W′ of the regression model under different pressures is compared with the measured value W.
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Table 1. Summary of basic gas parameters of 24 coal samples measured.
Table 1. Summary of basic gas parameters of 24 coal samples measured.
Coal Sample NumberSampling SiteMoisture
Mad/%
Ash
Aad/%
Volatile
Vdaf/%
True Density
TRD/(g·cm−3)
Apparent Density
ARD/(g·cm−3)
Porosity
k/%
Atmospheric Adsorption Capacity
Q/(cm3·g−1)
Gas Adsorption Constant
a/(cm3·g−1)
Gas Adsorption Constant
b/MPa−1
M01Xiangshan mine 3# coal seam 22301 return airway0.7926.8717.591.571.513.823.059524.59040.9459
M02Xiangshan Mine 5# coal seam track downhill0.9316.6714.261.481.433.383.432825.85051.1127
M0321220 mining face of 2# coal seam in Xiayukou Mine0.659.3616.201.391.343.603.019022.89601.1560
M04Xiayukou mine 3# coal seam 23306 Yunshun0.814.3014.441.321.292.273.352026.62490.9581
M0521301 open-off cut of 3# coal seam in Xinglong Coal Mine0.7011.7318.611.461.432.052.427617.05991.2944
M06Xinglong Mine 5# coal seam 4501 Yunshun0.6515.6417.901.501.453.333.128222.35451.251 5
M07Sangbei Mine 3# coal seam 11308 transport trough0.6812.0814.221.411.372.843.060519.77061.2854
M08Sangbei Mine 3# coal seam 11308 return air trough0.8210.0614.951.391.352.883.219522.77221.2786
M234301 control roadway of 3# coal seam in Sangshuping Mine0.739.6114.891.411.372.843.057022.41811.0547
M24South belt roadway of 3# coal seam in Sangshuping Mine0.8415.5315.201.481.442.703.736722.15341.5578
Table 2. Measured 24 coal samples relational model and other parameters summary table.
Table 2. Measured 24 coal samples relational model and other parameters summary table.
Coal Sample NumberSampling SiteInitial Velocity of Gas Diffusion Δp/mmHgConsistent Coefficient of Coal fK1p Relation Model(K1)p = 1WK1 Relation Model
M01Xiangshan mine 3# coal seam 22301 return airway210.49K1 = 0.5086 p0.57610.5086W = 5.408 lnK1 + 11.39
M02Xiangshan Mine 5# coal seam track downhill250.30K1 = 0.6598 p0.56520.6598W = 6.310 lnK1 + 11.94
M0321220 mining face of 2# coal seam in Xiayukou Mine200.32K1 = 0.4093 p0.61630.4093W = 6.053 lnK1 + 15.23
M04Xiayukou mine 3# coal seam 23306 Yunshun260.10K1 = 0.9097 p0.54270.9097W = 7.722 lnK1 + 11.35
M0521301 open-off cut of 3# coal seam in Xinglong Coal Mine140.22K1 = 0.4400 p0.65350.4400W = 4.000 lnK1 + 10.46
M06Xinglong Mine 5# coal seam 4501 Yunshun120.43K1 = 0.3438 p0.68710.3438W = 4.911 lnK1 + 14.35
M07Sangbei mine 3# coal seam 11308 transport trough140.39K1 = 0.2696 p0.61470.2696W = 5.015 lnK1 + 14.96
M08Sangbei mine 3# coal seam 11308 return air trough130.39K1 = 0.2704 p0.60400.2704W = 5.755 lnK1 + 17.00
M234301 control roadway of 3# coal seam in Sangshuping Mine100.44K1 = 0.2646 p0.66340.2646W = 5.271 nK1 + 12.04
M24South belt roadway of 3# coal seam in Sangshuping Mine160.31K1 = 0.2678 p0.71740.2678W = 4.368 lnK1 + 14.84
Table 3. Model summary.
Table 3. Model summary.
Regression ModelAdjusted R2SigDurbin-Wastson
(4)0.8330.0382.082
(5)0.6310.0011.377
Table 4. Comparison of predicted and measured values of the mathematical model of coal bed methane content.
Table 4. Comparison of predicted and measured values of the mathematical model of coal bed methane content.
Gas Pressure p/MPaXiayukou Coal Mine 23208 Working Face of 2# Coal SeamSangbei Coal Mine 3# Coal Seam 11308 Transport TroughXiangshan Coal Mine 5# Coal Seam South Wing Belt Transport Roadway
Measured Value (W)/(m3·t−1)Predicted Value (W′)/(m3·t−1)Error Rate/%Measured Value (W)/(m3·t−1)Predicted Value (W′)/(m3·t−1)Error Rate/%Measured Value (W)/(m3·t−1)Predicted Value (W′)/(m3·t−1)Error Rate/%
0.54.98363.7021−25.714.80444.1224−14.205.41555.48671.31
1.07.43375.7095−23.197.05956.1035−13.547.87197.5497−4.09
2.09.91047.7169−22.139.31718.0845−13.2310.28109.6128−6.50
3.011.20808.8912−20.6710.52929.2434−12.2111.556610.8196−6.38
4.012.04329.7243−19.2511.344610.0656−11.2712.409211.6758−5.91
5.012.649610.3760−17.9711.967210.7033−10.5613.058112.3400−5.50
Remarks: error rate = (W′–W)/W × 100%.
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Lei, H.; Dai, L.; Cao, J.; Li, R.; Wang, B. Experimental Study on Rapid Determination Method of Coal Seam Gas Content by Indirect Method. Processes 2023, 11, 925. https://doi.org/10.3390/pr11030925

AMA Style

Lei H, Dai L, Cao J, Li R, Wang B. Experimental Study on Rapid Determination Method of Coal Seam Gas Content by Indirect Method. Processes. 2023; 11(3):925. https://doi.org/10.3390/pr11030925

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Lei, Hongyan, Linchao Dai, Jie Cao, Rifu Li, and Bo Wang. 2023. "Experimental Study on Rapid Determination Method of Coal Seam Gas Content by Indirect Method" Processes 11, no. 3: 925. https://doi.org/10.3390/pr11030925

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