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Article

Detrital Zircon U-Pb Geochronology and Hf Isotope Geochemistry of the Hayang Group, SE Korea and the Himenoura and Goshoura Groups, SW Japan: Signs of Subduction-Related Magmatism after a Long Resting Period

1
Geology Division, Korea Institute of Geoscience and Mineral Resources, Daejeon 34132, Korea
2
Department of Earth and Environmental Sciences, Pukyong National University, Busan 48513, Korea
*
Author to whom correspondence should be addressed.
Minerals 2020, 10(11), 936; https://doi.org/10.3390/min10110936
Submission received: 1 September 2020 / Revised: 10 October 2020 / Accepted: 19 October 2020 / Published: 22 October 2020

Abstract

:
There was a hiatus in magmatism in Korea and Japan, located on the eastern continental margin of Asia, during a period of about 40 Ma from 160 Ma to 120 Ma. The cause of the resumption of magmatism since then is not yet well understood. In this study, we analyzed the Hf isotope composition of detrital zircons in the Cretaceous sediments of Korea (Hayang Group) and Japan (Goshoura and Himenoura groups) to investigate the tectonic evolution of eastern Asia in the Early Cretaceous period. εHf(t) in Cretaceous zircons from Japanese samples values from +8.2 to +0.1, suggesting that magmatism was sourced from the depleted juvenile materials, which is compatible with ridge subduction and subsequent melting of the young oceanic crust. εHf(t) values from Cretaceous zircons in the Hayang Group are negative, except for the Jindong Formation, which had a sediment supply from Japan, indicating that the old continental crust material of the Korean Peninsula was included in the magma generation. The detrital zircons of this study exhibit a depleted isotopic character at the beginning of subduction-related magmatism in Permian and Early Cretaceous, and then gradually change to a more enriched composition. This trend may be a typical example of the Pacific-type orogenic cycle.

1. Introduction and General Geology

The assembly of continental fragments in East Asia appears to have been completed during the Early Triassic period, when there was a continental collision between North China and South China blocks [1,2]. In the process of assembling continental fragments such as South China Block, North China Block, and Japanese Islands in this region, the Paleo-Pacific plates to the east have subducted below them and have triggered various tectonic activities and tectono-magmatic processes, including subduction-related magmatism [3,4,5], metamorphism [6,7,8], and terrestrial basin formation [9,10,11]. However, in the eastern margin of the Eurasia continent, especially in Japanese islands, igneous activities related to subduction of the Paleo-Pacific plate are observed even long before its complete assembly. The Japanese Islands have been affected by the subduction of Paleo-Pacific plates since about 500 Ma [12]. Since this time, there were several cyclic igneous activities called Pacific-type orogeny, and arc-related pull-apart sedimentary basins developed within the Japanese Islands [5,13]. As a result, the Japanese islands today consist mainly of tectonic units such as Paleozoic to Cenozoic accretionary complexes, high-pressure metamorphic belts, granite batholith suits, and sedimentary basins [5].
During the Phanerozoic subduction of Paleo-Pacific plates in the East Asian continental margin formed tectonic cycles repeated several times. It has been suggested that each cycle begins with an ocean ridge subduction (e.g., the Renge (Carboniferous), Farallon (Triassic), Izanagi (early Cretaceous), and Kula (late Cretaceous) [5]). The subduction of the Izanagi plate produced coeval Cretaceous orogenic components such as the Sanbagawa high-pressure metamorphic belt, the Sanbosan accretionary complex, the Ryoke-Sanyo batholith belt, and several sedimentary basins [13,14,15]. When each of these cycles begins and ends, and what characteristics do each of these cycles have over time is important in understanding these tectonic cycles. For example, the Mesozoic magmatism in Korea and Japan had a quiescent period from about 160 Ma to about 120 Ma [16,17,18].
The detrital zircons in sediments are suitable for studying the history of magmatism because they can comprehensively sample magmatism in the sediment source area and thus record the petrologic history of an arc. The detrital zircons of the Cretaceous basins of the Korean peninsula and Japanese islands, created by tectonic regime change during the Early Cretaceous period, are thought to be recording these changes in tectonic settings and magmatism [11,19,20]. The U-Pb age and Hf isotopic data of the detrital zircon can be used to trace the origin of the sediments, to limit the maximum deposition time, and to trace the tectonic environment and source materials of the magma-generated magma [21]. This study attempts to find out the temporal distribution of magmatism before the sedimentation by finding the distribution of U-Pb ages from the detrital zircons of the Cretaceous sediments in these regions, i.e., the Hayang Group in the southeastern Korean peninsula and Himenoura and Goshoura Group in SW Japan. From this, we verify the resumption period of early Cretaceous subduction-related magmatism, and also attempt to clarify the characteristics and tectonic settings of magmatism in that period through Hf isotope analysis of these zircons.
Sedimentary basins were produced in many places in Korea and Japan in the Cretaceous Period. The largest of these is the Gyeongsang Basin in the southeastern part of the Korean peninsula and consists of Sindong, Hayang, and Yucheon groups from the bottom. The Gyeongsang Basin was produced as a terrestrial back-arc basin [9]. No evidence of igneous activity in the early stages of basin formation was found, but detrital zircons with an age of about 128 Ma were found in the Nakdong Formation, the lowest layer, limiting the timing of basin formation [11]. Compared to the Sindong Group, where the detrital zircons of the Cretaceous age rarely appear, the overlying Hayang Group includes a high proportion of Cretaceous age zircons, especially those from about 120–110 Ma [19]. This indicates that there was enhanced igneous activity from this period and the tectonic environment gradually changed to intra-arc [19]. Cretaceous basins exist in several places in Southwest Japan. Among them, the Kanmon Group in Kyushu seems to have provenance of much of the sediment in the Korean Peninsula [22], suggesting that it was linked to Gyeongsang Basin at the time of deposition. The Cretaceous basins in Kyushu, unlike Korea, exhibit the characteristics of marine basins. However, there is evidence that sediments originated from the Korean Peninsula as detrital zircons include Paleoproterozoic ages, which are not present in Japan but characteristic of Precambrian basement rocks on the Korean Peninsula [22].
The Upper Cretaceous Himenoura Group and Geoshoura Group are distributed throughout the region including the Amakusa Islands, Kosikijima Islands, and the Uto Peninsulain in the western side of Kyushu (Figure 1) [23,24,25]. The basement rocks of Amakusa Island and the Uto Peninsula consist mainly of Cretaceous Higo plutonic-metamorphic rocks and Nagasaki metamorphic rocks [24]. The unconformably overlying rocks are composed of the Cretaceous Goshoura Group, Himenoura Group, Paleogene Miroku Group, Hondo Group, Sakasegawa Group, Neogene Kunhinotsu Group, and Paleogene to Neogene granitoids intruding into them. The Goshoura group is mainly distributed on the islands of Goshoura and Shishijima, which is the eastern part of the Amakusa Islands, and unconformably overlies the Higo Granitoids. The Goshoura Group is divided into Eboshi, Enokuchi, and Karakizaki formations in ascending order and consists of pebble bearing sandstone, sandstone and mudstone. Depositional environments of the Goshoura Group vary from terrestrial to marine deposits (e.g., floodplain, intertidal zone, and continental shelf) because of effects on sea-level fluctuation caused by repeated transgression and regression. Abundant mollusk fossils such as ammonite and bivalve have been reported from this group, suggesting that the sedimentation of the Goshoura Group ranges from Albian to Cenomanian [26,27].
The Himenoura Group extends from northeast to southwest and is exposed to the northeast of the Amakusa Islands. It is unconformable overlying the Higo plutonic and metamorphic rocks and the Goshoura Group and unconformably overlained by the Paleogene Miroku Group. The Himenora group is divided into lower subgroup and upper subgroup, the former consists of the lower Hinoshima Formation and the upper Amura Formation, and the latter consists of four formations from the U-I layer to the U-IV layer. Lower Hinoshima Formation is characterized by sedimentation of fining-upward sequences consisting of conglomerate, sandstone and mudstone, and upper Amura Formation is characterized by alternation of mudstone and sandstone. The Himenoura Group shows a variety of sedimentary environments from shallow marine to continental slopes and as well as pelagic deposits. In addition, the sedimentary environmental characteristics of the incised valleys have been reported from the lower part. Diverse fossils such as foraminiferas, radiolarians, ammonoids, and inoceramids have been found from the Himenoura Group, suggesting ages from Santonian to Campanian [28,29]. Recent zircon U-Pb age determination from felsic tuffs and suggested that the depositional ages of Hinoshima and Amura Formation were 85.4 ± 1.3 Ma (n = 15, MSWD = 0.83) and 81.5 ± 1.1 Ma (n = 20, MSWD = 1.3), respectively [25].
The Gyeongsang Basin is a Cretaceous non-marine sedimentary basin located southeast of the Korean peninsula (Figure 1). The west and north of the Gyeongsang Basin are surrounded by the Yeongnam Massif consisting of Paleoproterozoic metamorphic rocks and Mesozoic granitoids that intrude them. The east and south of the Gyeongsang basin face the sea. The Cretaceous Gyeongsang Supergroup deposited in the Gyeongsang basin consists of Sindong, Hayang, and Yucheon groups in ascending order [30]. The Hayang Group of the Miryang sub-basin is composed of Chilgok Formation, Silla Conglomerate, Haman Formation, and Jindong Formation in ascending order [31]. These formations were deposited in either alluvial, fluvial, or lacustrine environments [32]. In the lower layers of the Gyeongsang Basin, sediments were supplied by waters flowing from the west and northwest [33,34,35,36], but sediments constituting the upper layers were supplied from streams flowing from the east, the direction of the Japanese islands connected to the Korean Peninsula at the time [32,37,38,39]. The maximum depositional ages of the four formations constituting the Hayang Group defined from the youngest U-Pb age populations of detrital zircons are as follows; 109 Ma for the Chilgok Formation, 106 Ma for the Silla Conglomerate, 105 Ma for the Haman Formation, and 100 Ma for the Jindong Formation [19].

2. Samples and Analytic Methods

In this study, the hafnium isotopic compositions of detrital zircons were analyzed to study the characteristics of the subduction-related igneous activity resumed in the Cretaceous period. Therefore, samples were selected for sedimentary layers that are expected to have many detrital zircons of Cretaceous age. For the Gyeongsang Basin in Korea, we used the Hayang Group samples whose detrital zircon U-Pb ages have already been reported [19]; two in the Silla Conglomerate (Sila14, KU5) and one in each of the Chilgok (CG-1), Haman (HA-1), and Jindong (JD-2-1) Formations. For U-Pb age measurement and Hf isotope analysis, we used two sandstone samples from the upper Cretaceous Himenoura Group (Kuma-5, Kuma-6-1) and two samples from the mid Cretaceous Goshoura Group (Kuma-449 and Kuma-450), Kyushu, SW Japan, collected during the IGCP-507 field trip (Figure 1) [24]. Two samples of the Goshoura Group (Kuma-499, 450) were collected from a quarry on Goshoura Island. Sample Kuma-6 was collected from the lower Hinoshima Formation of the Himenoura group of the Uto Peninsula. The Kuma-5 sample was taken from the upper Amur Formation of the Himenoura Group on Kamishima Island.
U-Pb age determination of zircons separated from four samples of the Himenoura and Goshoura groups was conducted using Sensitive High-Resolution Ion Micro Probe (SHIRMP-IIe/Mc) operated by Korea Basic Science Institute (KBSI). For the SHRIMP U-Pb age determination, the O2 primary ion beam was used with diameter of about 25 μm and beam current of 2.0–4.0 nA. Zircon standards SL13 (U 238 ppm) and FC-1 (1099 Ma) [40] were used for uranium concentration and age calibration, respectively. All uncertainties for individual analysis points in the data table are quoted at one sigma level. Data reduction was performed using the SQUID 2.5 program [41]. Tera-Wasserburg diagrams, condordia ages, age histograms, and probability density plots were constructed using Isoplot 3.71 [42]. The 207Pb correction method was applied for 206Pb/238U ages below 1000 Ma, and the 204Pb correction method was applied for 207Pb/206Pb ages greater than 1000 Ma.
Hf isotope data for zircons were obtained from the same analysis spots as the U-Pb age measurements. Hf isotope composition was measured in KBSI using a Nu Plasma II multi collector inductively coupled plasma mass spectrometer equipped with a New Wave Research 193 nm ArF excimer ablation system (LA-MC-ICPMS). For Hf isotope analysis, 10 Faraday collectors were set up for simultaneous detection of Hf-Lu-Yb isotopes. Instrument parameters and operating conditions include spot size 50 μm, 10 Hz repetition rate, and energy density of 6–8 J/cm2. He (650 mL/min) and N2 (2 mL/min) were used as carrier gases for high Hf isotope intensity [43]. The spot depth in Hf isotope analysis is in the range of 15–30 μm. To monitor the measured isotope ratios, we used a time-resolved analytical (TRA) procedure. Signal intensities for each collector were collected every 0.2 s integration time. Background intensity, dwell time, and wash out time were measured for 35 s, 60 s, and 15 s, respectively. The isobaric interferences of 176Lu and 176Yb for the 176Hf signals were corrected using Chu et al. [44] and Vervoort, Patchett, Soderlund, and Baker [45]. The mass bias of the measured Hf isotope ratio was corrected to 179Hf/177Hf = 0.7325 using the exponential correction law [46]. All individual analyzes were calculated with 2-sigma uncertainty and data reduction was conducted with the Iolite 2.5 software program [47].

3. Results

3.1. U-Pb Age of the Detrital Zircons from the Himenoura and Goshoura Groups

Most of the detrital zircons separated from the sandstones of the Himenoura Group and the Goshoura Group of SW Japan except for one sample (Kuma-5) have crystal shapes of euhedral to subhedral with well-developed oscillatory growth zoning with no evidence of pre-Cretaceous zircon or old cores in CL images (Figure 2).
The U-Pb ages for 90 analytical spots for 85 zircon grains from the Himenoura Group and Goshoura Group of SW Japan are shown in Table A1 and Figure 3. Most zircon grains yield concordant or slightly discordant U-Pb ages. In the samples other than one (Kima-5), each single concordia age was obtained. The two samples of the Goshoura Group (Kuma-449, 450) yield concordia ages of 110.3 ± 0.7 Ma (n = 32, MSWD = 3.1) and 116.8 ± 0.8 Ma (n = 15, MSWD = 2.6), respectively. The lower Hinoshima Formation sample (Kuma-6) of the Himenoura group yields a concordant age of 114.9 ± 0.9 Ma (n = 12, MSWD = 1.4). Unlike these, the upper Amura Formation sample (Kuma-5) of the Himenoura group yields a wide range of ages from ca 2360 Ma to 86 Ma. The concordia ages of 88.4 ± 1.3 Ma (n = 6, MSWD = 0.1), 95.8 ± 1.6 Ma (n = 4, MSWD = 1.2), and 254.3 ± 1.8 Ma (n = 3, MSWD = 1.2) were obtained from the sample Kuma-5. Of the four samples analyzed from the Himenoura Group and Goshoura Group, only Kuma-5 has detrital zircons with ages other than Cretaceous, including Jurassic, Triassic, Permian, and Paleoproterozoic ones (Figure 4).

3.2. Hf Isotopic Compositions of the Detrital Zircons from the Goshoura and Himenoura Groups, SW Japan

The analyzed Hf isotope compositions of the detrital zircons from the Goshoura Group and Himenoura Group in SW Japan are listed in Table A2. Of the four samples from the Goshoura Group and Himenoura Group, three with similar concordia ages of about 110–115 Ma exhibit positive εHf(t) values of +8.5 to +3.6 except for one analysis spot (Kuma-450-3.1) with a value of -7.8 (Figure 5). Their T2DM age ranges from 842 Ma to 560 Ma, and the exceptional spot (Kuma-450-3.1) has an older T2DM age of 1469 Ma. Sample Kuma-5, however, shows a wide range of εHf(t) values (+9.3 to −21.1) and T2DM ages (580 Ma to 2805 Ma). Among them, the εHf(t) values of the Cretaceous zircons are divided into two groups: +8.2 to +0.1 and −14.7 to −21.1. Jurassic zircon of Kuma-5 has an εHf(t) value of −19.6 and a T2DM age of 2163 Ma. From late Permian to Triassic, zircons have εHf(t) from +9.3 to +2.6, and Precambrian zircons range from +3.4 to −3.3.

3.3. Hf Isotopic Compositions of the Detrital Zircons from the Hayang Group, Korea

In this study, Hf isotope composition was also analyzed from detrital zircons of Hayang Group in Gyeongsang basin, Korea (Table A3), which had already analyzed U-Pb ages [19]. The detrital zircons of the Hayang Group have a much wider range of U-Pb ages [19] than those of the Goshoura and Himenoura groups. The εHf(t) values of detrital zircons of the Hayang Group show significant changes with geological age. The Cretaceous detrital zircon grains mostly preserve the euhedral shape with sharp crystal edges, but the older zircon grains tend to develop roundness (Figure 4). In the case of Cretaceous zircons, which are almost half of all zircons, the εHf(t) value varies from −27.0 to +9.3 (Figure 5). Interestingly, negative εHf(t) values appear in all the lower three formations of the Hayang Group, and positive values appear only in the Jindong Formation at the top. The εHf(t) of the Jurassic and Triassic zircons ranges from −22.3 to −5.4. In the Jindong Formation, unlike other formations, a large number of Permian zircons appear and have fairly high positive εHf(t) values from +11.0 to +13.8. The Paleoproterozoic and Archean zircons of the Hayang Group show εHf(t) values of −32.9 to +7.0 (Figure 5). The Neoproterozoic and Mesoproterozoic zircons of the Hayang Group have a significant range of the εHf(t) values from −30.3 to +18.2.

4. Discussion

4.1. Provenance of Detrital Zircons of the Goshoura and Himenoura Groups

The detrital zircon grains of the three of the four samples from the Goshoura and Himenoura groups (Kuma-499, Kuma-450, and Kuma-6) show euhedral to subhedral shapes with well-preserved crystal edges instead of showing well developed roundness indicating the relatively short sediment transport distance (Figure 2). These samples yield single concordia ages with small errors of 110.3 ± 0.7 Ma, 116.8 ± 0.8 Ma, and 114.9 ± 0.9 Ma, respectively. The Th/U ratios of these zircons (0.25–0.96) are larger than 0.1, which is a general criterion that distinguishes igneous zircons from metamorphic zircons [50]. Therefore, it is presumed that these relatively homogeneous detrital zircons originate from igneous protoliths not far away. In contrast to these, the detrital zircon grains separated from the upper Amura Formation (Kuma-5) of the Himenoura group show a wide range of age distributions and the degree of development of roundness of grains. Among the zircon grains of the sample Kuma-5, Cretaceous ones have euhedral shapes like other samples. However, the older zircon grains show relatively rounded edges. In particular, the Paleoproterozoic zircon grains have more developed roundness (Figure 2c). Although the roundness of detrital zircon grains is not a definite quantitative measure of transport distance, it appears to reflect the degree of age variance and relative transport distance in the analyzed samples. All the analyzed zircons from Kima-5 have Th/U ratios greater than 0.1, implying igneous origin. The youngest concordia ages in the Goshoura Group and the Himenoura Group are 110.3 ± 0.7 Ma and 88.4 ± 1.3 Ma, respectively, somewhat older than previously reported fossil ages [26,27,28,29]. Recently, a slightly younger age of 81.5 ± 1.4 Ma was reported from the upper part of the Amura Formation and was suggested as the maximum depositional age [25]. Thus, these Cretaceous zircons were reworked from existing rocks or sediments and are not the product of syn-sedimentary volcanic activity. Among the detrital zircons of sample Kuma-5, the proportion of Paleoproterozoic is about 45%.
The U-Pb concordant ages calculated from detrital zircons of the Goshoura Group and Himenoura Group were 114.9 ± 0.9 Ma, 111.6 ± 0.8 Ma, 110.3 ± 0.7 Ma, 95.8 ± 1.6 Ma, and 88.4 ± 1.3 Ma. The U-Pb ages of the granitoids of the Higo metamorphic belt, the basement rock of Goshoura and Himenoura Groups, were reported from ca. 117 Ma to 108 Ma [51,52]. These Cretaceous ages of the Higo belt are consistent with the detrital zircon ages of the Goshoura and Himenoura groups with concordia ages of about 115 Ma to 110 Ma. Accordingly, the Higo belt is inferred as the main source of the Cretaceous detrital zircons of about 115–110 Ma deposited in Goshoura and Himenoura Groups. However, the U-Pb age of Amura Formation (Kuma-5), the upper layer of the Cretaceous Himenora group, shows ages between 2357 Ma and 86 Ma. More than 45% of these consist of Paleoproterozoic zircons, showing a different age distribution pattern than the other three samples. Although the Paleoproterozoic zircons should have been derived from the old continental crust, rocks of that age have not yet been reported on the Japanese Islands. However, on the Korean peninsula close to Japan, Paleoproterozoic rocks [53,54] corresponding to the zircon ages of Kuma-5 are exposed to the surface in a large area. Given the interconnection of the Korean Peninsula and the Japanese Islands before the opening of the East Sea (Sea of Japan) in Cenozoic [55], the presence of these Paleoproterozoic zircons indicates the supply of sediments from the inland area, presumably the current Korean Peninsula. We suggest that the basin-fills from the middle to the upper-middle part of the Cretaceous Basin in the Amakusa Islands were initially supplied primarily from source rocks in the nearby Higo belt where Cretaceous igneous rocks of similar age are distributed. However, the sediments of the Amura Formation were supplied from sources within the nearby Higo belt as well as from the distant inland areas.
The sample Kuma-5 of the Himenoura Group also yielded a Permian concordant age of 254.3 ± 1.8 Ma. In fact, Permian igneous rocks have been found in several areas of Japan, including the nearby Kyushu area. The Usukigawa granodiorite, located in east central Kyushu, has a zircon U-Pb age of ca. 290 Ma [52]. The Kinshozan Quartz Diorite from the Kanto Mountains, Japan, has a zircon U-Pb age of 281.5 ± 1.8 Ma [56]. Permian zircon U-Pb ages of 292 to 259 Ma have been reported from granitoids in the Maizuru area [57]. A new U–Pb zircon geochronological study for the paragneisses from the Tateyama area in the Hida Mountains of north central Japan showed that the detrital zircons had a core age of about 275 Ma and overgrowth ages due to metamorphism of around 235–250 Ma [58]. However, in the case of the Himenoura Group, considering that Th/U ratios of all zircons are greater than 0.1 implying igneous origin, it is suggested that Permian igneous rocks from other regions than the paragneiss of the Hida Mountains were the source of the studied detrital zircons.
Hf isotopic compositions of the detrital zircons are also helpful in tracking the provenance of sediments. The εHf(t) values of the Jurassic and Triassic zircons of the Hayang Group ranges from −18.2 to −5.4 and agree well with typical values for Jurassic and Triassic granitoids known in South Korea [59,60]. The Paleoproterozoic and Archean zircons of the Hayang Group have εHf(t) values of −14.8 to +6.9 and are similar to the Paleoproterozoic basement rocks of the Yeongnam massif surrounding the Gyeongsang basin [54,61]. The Neoproterozoic and Mesoproterozoic zircons of the Hayang Group appear to have been derived from the Okcheon metamorphic belt in the northwest [19]. During this period, the εHf(t) values of zircons show a significant range of changes from −30.3 to +18.2. The lower values appear to follow the evolution curve of the Archean continental crust, like the Paleoproterozoic and Archean zircons (Figure 5). However, some higher values seem to reflect the input of juvenile material from the depleted mantle at the time. This is consistent with the high εHf(t) values reported from constituent members of the Okcheon metamorphic belt, reflecting rifting events related to breakup in supercontinent Columbia during the Mesoproterozoic [62].

4.2. Resumption of Igneous Activities at about 120 Ma after a Break for 40 Ma

In the Korean peninsula and Japanese islands located at the eastern margin of the Eurasia continent, there was a long resting period without active magmatism from about 160 Ma to about 120 Ma [16,17,18]. Therefore, in the detrital zircons of the Cretaceous basins of these regions, ages during this long magmatic gap are hardly found. In the Nakdong Formation, the lowermost part of the Cretaceous Gyeongsang basin in the southeastern part of the Korean Peninsula, about 128 Ma of igneous zircons were found [11]. This age marks the beginning of the deposition of the Nakdong Formation, that is, the beginning of the development of the Cretaceous Gyeongsan basin. The igneous rock of this age has not yet been discovered in the Korean Peninsula, but granitoids of about 130–110 Ma are widely exposed in the Kitakami zone in Northeast Japan [63,64]. The emergence of granitoid plutons of this age in the Japanese islands indicates the resumption of igneous activity after a similar magmatic gap on the Korean Peninsula.
In the detrital zircons of the Himenoura Group and the Goshoura Group in southwestern Japan and the Hayang Group in the southeastern Korean peninsula, zircons of about 120–110 Ma, which are about 10–20 Ma younger than the Nakdong Formation, are common. Both the Korean peninsula and the Japanese islands, igneous rocks of this range of age are more common than those of about 120–130 Ma. Granitoids of 109–114 Ma are distributed in the southwestern part of North Korea [65]. In the western and central regions of the Gyeonggi massif in South Korea, igneous activities of about 110 Ma have been reported [66]. In Southwest Japan, several plutonic rocks in the central Kyushu region have zircon U-Pb ages of 108–117 Ma: Oshima quartz dioritic gneiss, Oshima granitic gneiss, Ryuhozan gabbro, Miyanohara tonalite, and Mansaka tonalite [51,52]. Zircon U–Pb ages of plutonic rocks in the southern Abukuma Mountains of Northeast Japan indicate that the intrusion ages of gabbroic rocks and surrounding granitic rocks ranges from 113 to 100 Ma [67]. Taken together, it seems that the long paused magmatism has resumed at about 130 Ma in the Kitamami zone in Northeast Japan. However, in a wide area extending to Southwest Japan and the Korean Peninsula, there seems to have been active magmatism at about 120–110 Ma a little later.

4.3. Input of Juvenile Mantle Material with Resumption of Magmatism

The detrital zircon of igneous origin retains the original hafnium isotopic value of the melt from which it was crystallized without post-crystallization radiogenic growth due to the low Lu/Hf ratio. Therefore, the Hf isotope values of detrital zircons are suitable for examining tectonic environment related to magmatism in their provenance [21,68]. The results of this study and the age distribution of Cretaceous granitoids in Korea and Japan show that there was a very active igneous activity from about 130–120 Ma after a magmatic gap of 30–40 Ma beginning at about 160 Ma. The Hf isotope composition in the detrital zircons of this period are characterized bimodal εHf(t) values of quite positive and significant negative values. Among the analysis results, most of the Cretaceous zircons of the Goshoura and Himenoura groups in Japan have positive εHf(t) values, but in the case of the Hayang Group on the Korean Peninsula, on the contrary, the Cretaceous zircons of the other formations except the Jindong Formation show negative values. Among these positive Cretaceous zircons are discussed first, and other results are discussed later.
The Mesozoic granitoids of the SW Japan mostly have εNd(t) values in the range of −15 to +5 and an average value of about −4, which is interpreted to have a source rock containing a large amount of recycled continental crust [69]. However, the Early Cretaceous detrital zircons of the Goshoura and Himenoura groups have a more depleted value of positive εHf(t), so it is necessary to investigate the cause. In general, high εHf(t) values indicate origin from depleted mantle or juvenile young oceanic crust, while low εHf(t) values represent origin from old continental crust sources [70]. Therefore, the positive εHf(t) of the Early Cretaceous zircons of the Goshoura and Himenoura groups represents the input of juvenile materials from the depleted mantle. Meanwhile, Early Cretaceous granitoids in the Kitakami zone in Northeast Japan have positive εHf(t) values [63] that are similar to or slightly higher than the Cretaceous detrital zircons in this study (Figure 5). Early Cretaceous Kitakami granitic plutons have been suggested to include rocks of adakitic affinity and mostly derived from juvenile oceanic crustal sources [64]. The generation model of adakitic magma includes the melting of young oceanic crusts or the melting of eclogite created by underplating these oceanic crusts underneath the crust [71,72,73,74]. The melts generated in this way may contain juvenile materials derived from depleted mantle in a high proportion, and thus the εHf(t) value may be quite high [75].
During the early Cretaceous period of 120–110 Ma, numerous igneous rocks were emplaced over large areas of Japan, including, for example, Ryoke-Sanyo batholith and a number of numerous granitoids distributed in the Abukuma belt, Sikoku area, and Higo belt [51,52,63,64,65,66,67]. Particular attention should be paid to the granitoids of Abukuma and Higo belts. These granitoids have zircon U-Pb ages ranging from 118 Ma to 101 Ma and exhibit the geochemical characteristics of adakite formed by slab melting of young oceanic crusts (e.g., Shiraishino adakitic pluton [76]). Recently, Maki et al. [51] conducted U-Pb age determination and Hf isotope analysis of diatexitic migmatite on Higo belts and obtained an age of 110.1 ± 0.6 Ma (n = 11, MSWD = 1.10) and high εHf(t) values up to +11.8. They also argued that the presence of diatexitic migmatite with high εHf(t) values reflects the influence of the highly depleted mantle and juvenile components, and may be related to the remelting of basalt produced from the depleted mantle. Coeval igneous rocks affected by depleted mantle-derived juvenile components have also been reported in Abukuma, in northeastern Japan. Tsuchiya et al. [64] claimed that the Cretaceous Abukuma granite had an age of 118–117 Ma and the geochemical characteristics of adakite. Therefore, the inclusion of juvenile mantle materials in magmatism that resumed after a long resting period was confirmed not only in detrital zircons in sedimentary formations in Southwest Japan, but also in 120–110 Ma granitoids in Northeast Japan.

4.4. Negative εHf(t) Values of Cretaceous Zircons

The εHf(t) values of the Cretaceous detrital zircons analyzed in this study show a bimodal distribution pattern that is divided into a fairly positive group and a significantly negative group. The positive group appears in Himenoura and Goshoura groups and Jindong Formation, and the negative group appears mainly in Chilgok, Silla, and Haman formations (Figure 5). That is, the positive group appears mainly on the Japanese side, and the negative group appears mostly on the Korean side, except for some zircons of Jindong Formation. One thing to note here is that when Jindong Formation was deposited, the flow direction of paleocurrent indicates the supply of sediment from the east, or the Japanese side [32,37,38,39]. Therefore, the detrital zircons of the positive group appearing in Jindong Formation may originate from sediment sources in Japan. Considering this, it suggests that the igneous activities at that time had the characteristics of mainly positive εHf(t) in the vicinity of the trench and significantly negative εHf(t) in the inland side. The fairly low εHf(t) values in the inland indicate that magma genesis and differentiation processes were affected by old crustal materials below the Korean Peninsula. A similar range of negative εHf(t) values can be seen in the Triassic to Jurassic igneous rocks of the Korean Peninsula [60]. This characteristic also appears in the εHf(t) values of the Triassic to Jurassic detrital zircons (−5 to −25) included in sedimentary layers of the Hayang Group (Figure 5) reflecting the influence of materials from the old continental curst of the Korean Peninsula.

4.5. Variability of εHf(t) Values Over Time

The high εHf(t) values of about 120–110 Ma detrital zircons are somewhat different from those previously reported from the Cretaceous to Paleogene granitoids from Southwest Japan. For example, the granitic rocks in the Iwakuni area in Southwest Japan have a zircon U-Pb age of 104–92 Ma and εHf(t) in the range of −5 to +0.7 [77]. The results of Sr-Nd isotope analysis for Phanerozoic granitoids from Southwest Japan generally show negative εNd(t) values and high initial 87Sr/86Sr ratios [69]. Therefore, it is clear that there was a temporal change from the high εHf(t) values of Early Cretaceous to the lower values of the later period. When ridge subduction occurs, the volume of the melting zone may be larger because of the enhanced temperature, and continental materials in the lower crust may be added to the melt. The magma formed in the later stages through this process may have a larger proportion of enriched materials compared to the earlier ones mainly derived from the young oceanic crust.
However, the temporal change of isotope values from depleted values to more enriched values does not appear only in the Cretaceous period. It is known that there was Permian igneous activity in both Korea and Japan, and it seems that there was no magmatism for a long time before that. The Permian zircons (270–300 Ma) of the Jindong Formation, which originated in Japan, show that the εHf(t) values of Permian granitoids appearing after the dormant period of magmatism are quite high, ranging from +11 to +14 (Figure 5). The Yeongdeok granite, located in the east-central part of the Korean peninsula at about 260 Ma, slightly younger than the Permian zircons of the Jindong Formation, also has adakitic characteristics and at the same time has an εHf(t) value of about +11.5, depleted isotopic composition [60]. In the Hayang Group, the εHf(t) values of Triassic to Jurassic detrital zircons also show a shift toward more enriched isotope composition than those of Permian (Figure 5). The tectonics of repetitive changes in the εHf(t) values in the Pacific type of orogenic cycle are outside the scope of this study, but it is worth noting.

4.6. Since Early Cretaceous, Japanese Islands Have Moved 1000 km Northeast from Next to South China?

Researchers of the Kitakami adakites argue that the magmatism of the time was caused by ridge subduction that migrated northward, and that these plutons were translated northeastward more than 1000 km from their original location next to South China [5]. However, considering the relationship with neighboring blocks, such a long-distance movement is not very persuasive and seems not necessary. First of all, there seems to be no significant difference in the history of tectonic evolution between Northeast Japan and Southwest Japan. One of the characteristics of Northeast Japan is the existence of Early Paleozoic plutons, which are about 500–450 Ma [12,56]. However, evidence of igneous activity in the Paleozoic era corresponding to this period was also found in Southwest Japan. The LA-ICP-MS zircon U–Pb geochronology revealed that the intrusion age of Saganoseki quartz diorite was 473.3 ± 3.6 Ma [78].
Early Cretaceous tectonic environments also appear to be similar in Northeast and Southwest Japan. The resumption of subduction-related igneous activity after a long resting period can be determined by the age of about 130–110 Ma granitoids that occur in various parts of Japan and by the age distribution patterns of detrital zircons in sediments. In the case of Northeast Japan, the age of plutons intruded in the Kitakami zone includes those of about 130–120 Ma. In the case of Southwest Japan, the maximum age of Early Cretaceous plutons or detrital zircons is about 120 Ma, suggesting that igneous activity may have begun in Northeast Japan slightly earlier than in Southwest Japan. However, both regions are similar in that the restarted magmatism has a high hafnium initial isotopic composition, indicating the melting of the material derived from the young oceanic crust. Since the resumption of magmatism was almost the same and the properties of the source material were similar, it is highly likely that the two regions shared the same tectonic setting. Several evidences have suggested that Southwest Japan and the Korean Peninsula were connected to each other in the Early Cretaceous period [55]. In particular, the research shows that during the Cretaceous period sediment was supplied from Japan to Korea and from Korea to Japan, depending on the location, supporting this [19,22,23,79]. This connection between Southwest Japan and the Korean Peninsula in Early Cretaceous contradicts the suggestion that Northeast Japan or the whole of Japan is located next to south China in Early Cretaceous and moved about 1000 km northeast to its present location.

5. Conclusions

Most of the detrital zircons of the Goshoura and Himenoura groups in west central Kyushu in Southwest Japan have U-Pb ages in the Cretaceous period, but some have older Permian or Paleoproterozoic ages. The detrital zircons with Paleoproterozoic ages indicate sediment supply from the inland area, possibly from the Korean Peninsula that was connected during their deposition. The Cretaceous age of about 120–110 Ma indicates that magmatism resumed after the previous dormant period, and the Japanese zircons have quite positive εHf(t) values. These detrital zircons, which appear to have originated from the igneous rocks of Southwest Japan, are likely to have been produced by ridge subduction that led to the melting of the young oceanic crust. We suggested that later Japanese granitoids generally show a more enriched isotope composition as a result of the melting of a wider volume as the ridge subduction proceeds and contain more crust components. All of the Cretaceous zircons of the Hayang Group have quite negative εHf(t) values, except for the Jindong Formation, which had a sediment supply from Japan. This is interpreted as the fact that the old continental crust material on the Korean Peninsula was included in the magma generation. The subduction-related magmatism started in Permian shows the characteristics of adakite generation and high εHf(t) value. Meanwhile, the composition of subsequent magmatisms changed to more enriched. This repetitive trend of change can be a typical example of the Pacific-type orogenic cycle.

Author Contributions

Conceptualization, T.-H.L. and K.-H.P.; methodology, K.-H.P.; validation, T.-H.L. and K.-H.P.; formal analysis, T.-H.L.; investigation, K.-H.P.; writing—original draft preparation, K.-H.P.; writing—review and editing, K.-H.P.; visualization, T.-H.L.; supervision, K.-H.P.; funding acquisition, K.-H.P. All authors have read and agreed to the published version of the manuscript.

Funding

This work was supported by the National Research Foundation of Korea (NRF) grant funded by the Korea government (MSIT) (No. NRF-2019R1A2C2002506). This research was also supported by a grant (GP2020-014) from the Research in Active Tectonics and Development of Fault Segmentation Model for Intraplate regions from Basic Research Project of the Korea Institute of Geoscience and Mineral Resources (KIGAM) funded by the Korean Ministry of Science and ICT.

Acknowledgments

We would like to thank Komatsu who organized and guided fourth international symposium and field trip of the IGCP507. We deeply appreciate the meticulous and constructive opinions of the anonymous reviewers.

Conflicts of Interest

The authors declare no conflict of interest. The funders had no role in the design of the study; in the collection, analyses, or interpretation of data; in the writing of the manuscript, or in the decision to publish the results.

Appendix A

Table A1. SHRIMP U-Pb results for the detrital zircons from the Goshoura and Himenoura Groups, Southwest Japan.
Table A1. SHRIMP U-Pb results for the detrital zircons from the Goshoura and Himenoura Groups, Southwest Japan.
Spot No.U (ppm)Th (ppm)Th/UCommon 206Pb (%)238U/206Pb± (%)207Pb/206Pb± (%)Apparent Age (Ma)
Kuma-449
Kuma-449-1.12241030.480.0057.01.60.061114.8110.3 ± 1.3
Kuma-449-2.12471180.500.0658.61.80.041220.5110.1 ± 1.6
Kuma-449-2.22341110.490.3758.21.80.066211.8107.3 ± 1.7
Kuma-449-3.1105690.680.0060.42.70.046139.9106.1 ± 1.5
Kuma-449-4.13212120.680.2058.02.20.058011.0108.9 ± 2.2
Kuma-449-5.15962620.450.0059.21.80.04319.9108.6 ± 1.9
Kuma-449-6.1208980.490.0058.72.40.055214.4107.9 ± 2.4
Kuma-449-7.15082110.430.0960.01.30.05195.6106.1 ± 1.3
Kuma-449-8.12891280.460.0057.72.00.034119.7112.8 ± 2.1
Kuma-449-9.14292480.600.0057.21.10.04478.9112.3 ± 1.1
Kuma-449-10.1206850.430.5659.01.90.045717.8108.7 ± 1.8
Kuma-449-11.12191450.680.0058.01.50.053616.6109.5 ± 1.2
Kuma-449-12.1122530.450.0356.21.90.059719.8112.0 ± 1.4
Kuma-449-13.110065330.550.0757.90.90.04805.3110.5 ± 1.0
Kuma-449-14.1265950.370.0057.22.10.053712.7110.9 ± 2.1
Kuma-449-15.14282020.490.0059.31.30.04358.6108.3 ± 1.4
Kuma-449-16.11981480.770.0058.71.90.052417.9108.4 ± 1.7
Kuma-449-17.110597510.730.0057.61.20.04823.0111.0 ± 1.3
Kuma-449-18.1203940.485.2356.81.80.051123.7112.1 ± 1.2
Kuma-449-19.12421230.530.2857.41.90.059712.7109.7 ± 1.8
Kuma-449-20.13272160.680.0058.31.80.05809.5108.2 ± 1.8
Kuma-449-21.1100580.600.0057.23.70.068829.1108.9 ± 3.0
Kuma-449-22.13782030.560.3757.21.90.05038.7111.4 ± 2.0
Kuma-449-23.12271130.510.0756.31.80.055014.7112.5 ± 1.7
Kuma-449-24.12261510.690.0258.21.90.052913.8109.3 ± 1.9
Kuma-449-25.1178970.560.0059.72.00.043729.7107.7 ± 1.3
Kuma-449-26.1133710.550.0055.83.00.074116.7110.8 ± 2.8
Kuma-449-27.117548390.490.3258.41.00.05032.8109.1 ± 1.1
Kuma-449-28.13061970.670.0057.82.20.042618.0111.3 ± 2.3
Kuma-449-29.182400.500.0054.94.40.054341.0115.5 ± 3.9
Kuma-449-29.21501150.790.0756.41.90.056221.7112.1 ± 1.5
Kuma-449-30.1160790.510.1357.43.50.064121.2109.2 ± 3.4
Kuma-450
Kuma-450-1.15393080.590.0756.81.00.04367.8113.1 ± 1.1
Kuma-450-1.22101030.510.0056.02.20.052312.0113.5 ± 2.3
Kuma-450-2.15633640.670.0057.41.40.04896.5111.3 ± 1.6
Kuma-450-3.11341010.780.0059.72.40.038338.8108.4 ± 1.7
Kuma-450-4.110726520.630.0956.90.90.04943.1112.1 ± 1.0
Kuma-450-5.19073980.450.3057.51.60.05033.4110.9 ± 1.8
Kuma-450-6.13241780.570.1756.31.50.04679.4113.8 ± 1.6
Kuma-450-7.12631960.770.0056.61.60.047111.9113.0 ± 1.7
Kuma-450-8.1232112470.550.3257.10.90.04881.8111.9 ± 0.9
Kuma-450-9.18715280.630.0256.51.30.04973.7112.9 ± 1.4
Kuma-450-10.18625090.610.2058.81.60.05224.6108.1 ± 1.7
Kuma-450-11.110278170.820.0058.31.10.04954.8109.5 ± 1.2
Kuma-450-12.12371300.570.1757.31.60.048514.4111.5 ± 1.5
Kuma-450-13.1145890.630.0059.32.40.047223.8107.9 ± 2.4
Kuma-450-14.11551100.730.1258.51.60.049720.5109.1 ± 1.2
Kuma-5
Kuma-5-1.17064130.601.342.90.90.12900.42084.6 ± 6.6
Kuma-5-1.294680.750.762.71.30.13141.12116.6 ± 19.0
Kuma-5-2.1128590.480.0073.84.30.052038.186.3 ± 3.1
Kuma-5-3.12871590.570.062.51.00.13340.62142.9 ± 10.2
Kuma-5-4.17593330.450.0466.71.00.05117.095.6 ± 0.9
Kuma-5-5.1325330.100.002.91.60.11510.61882.2 ± 11.3
Kuma-5-6.11421040.750.222.51.20.13910.92216.1 ± 14.8
Kuma-5-7.14161490.370.0066.02.10.051111.696.5 ± 1.9
Kuma-5-8.1324870.280.093.01.50.11500.61879.6 ± 11.4
Kuma-5-9.1162613790.883.904.01.30.11390.61862.6 ± 11.7
Kuma-5-10.14531980.450.002.41.10.13680.42186.9 ± 6.5
Kuma-5-11.18631500.180.063.01.10.11380.31861.7 ± 5.8
Kuma-5-12.17756030.805.0767.42.50.055715.094.0 ± 2.1
Kuma-5-13.1120870.742.6670.94.40.057535.889.2 ± 3.2
Kuma-5-14.11361040.790.0072.83.30.061328.686.5 ± 2.2
Kuma-5-15.15794380.780.0074.71.50.04567.986.0 ± 1.2
Kuma-5-16.11881941.060.0068.83.00.039628.594.0 ± 2.6
Kuma-5-17.1657880.141.743.31.30.11700.81910.3 ± 15.2
Kuma-5-18.18802580.300.0824.50.90.05202.2257.6 ± 2.4
Kuma-5-18.220136180.320.3225.51.10.05201.5247.6 ± 2.8
Kuma-5-19.14202340.580.2673.73.00.050210.386.7 ± 2.6
Kuma-5-20.17502910.400.1139.11.20.04913.6162.9 ± 1.9
Kuma-5-21.11601040.670.0056.52.90.053920.6112.3 ± 2.9
Kuma-5-22.1221920.430.003.01.10.11480.71876.4 ± 13.1
Kuma-5-23.12091110.550.1053.71.40.051814.1118.4 ± 1.4
Kuma-5-24.15584190.780.1629.61.60.04934.7214.8 ± 3.3
Kuma-5-25.1126013321.090.1171.50.90.04724.489.6 ± 0.8
Kuma-5-26.12572180.880.002.41.90.13480.62161.0 ± 9.9
Kuma-5-27.1116580.510.622.31.20.15090.82356.5 ± 13.9
Kuma-5-28.1267500.190.002.91.00.11520.71883.4 ± 12.3
Kuma-5-29.135230.670.1724.33.30.077428.3251.2 ± 4.7
Kuma-6
Kuma-6-1.18283420.430.1855.41.30.05112.5114.9 ± 1.5
Kuma-6-2.111062640.250.0256.20.90.04881.8113.7 ± 1.0
Kuma-6-3.110492700.270.0156.50.90.04831.9113.1 ± 1.0
Kuma-6-4.16143610.610.1555.40.90.04713.5115.6 ± 1.1
Kuma-6-5.113203330.260.0654.91.40.04782.1116.4 ± 1.7
Kuma-6-6.12971440.500.0055.31.40.04416.5116.1 ± 1.6
Kuma-6-7.17181760.250.0056.70.90.04543.8113.1 ± 1.1
Kuma-6-8.1234940.420.2755.52.40.039017.1116.6 ± 2.7
Kuma-6-9.1190811580.630.1354.80.90.04871.5116.5 ± 1.0
Kuma-6-10.110579810.960.0056.00.90.04751.7114.3 ± 1.0
Kuma-6-11.14961590.330.1258.21.50.04604.5110.1 ± 1.6
Kuma-6-12.110302400.240.0054.31.00.04552.6118.0 ± 1.2
Table A2. LA-MC-ICPMS Lu-Yb-Hf isotopic compositions of the detrital zircons from the Goshoura and Himenoura Groups, Southwest Japan.
Table A2. LA-MC-ICPMS Lu-Yb-Hf isotopic compositions of the detrital zircons from the Goshoura and Himenoura Groups, Southwest Japan.
Spot No.176Hf/177Hf±2 S.E.176Lu/177Hf±2 S.E.176Yb/177Hf±2 S.E.εHf(t)T2DM (Ma)
Kuma-449
Kuma-449-1.10.2829180.0000220.0010030.0000330.026400.001107.5618
Kuma-449-2.10.2828780.0000210.0013830.0000360.037270.000746.1699
Kuma-449-2.20.2829120.0000190.0005430.0000050.013540.000237.3629
Kuma-449-3.10.2829130.0000220.0008840.0000150.027760.000477.3629
Kuma-449-4.10.2828900.0000200.0009190.0000150.026780.000586.5674
Kuma-449-5.10.2828780.0000230.0008340.0000080.022040.000236.1697
Kuma-449-6.10.2829190.0000230.0004990.0000070.012130.000297.5615
Kuma-449-7.10.2829210.0000290.0016990.0000740.050800.002307.5616
Kuma-449-8.10.2828780.0000240.0013110.0000400.037000.000946.1698
Kuma-449-9.10.2828890.0000190.0007440.0000080.019270.000116.5674
Kuma-449-10.10.2828960.0000190.0005920.0000050.016420.000176.7661
Kuma-449-11.10.2829240.0000210.0007600.0000050.020490.000317.7605
Kuma-449-12.10.2828890.0000210.0007880.0000230.020790.000466.5674
Kuma-449-13.10.2828960.0000280.0018480.0000470.052600.001506.7665
Kuma-449-14.10.2829060.0000250.0011020.0000190.029690.000897.1642
Kuma-449-15.10.2828880.0000210.0009610.0000100.025680.000236.4678
Kuma-449-16.10.2829110.0000260.0009280.0000200.024580.000417.2632
Kuma-449-17.10.2829010.0000270.0020260.0000220.057050.000626.8656
Kuma-449-18.10.2829140.0000190.0005970.0000150.016560.000477.4624
Kuma-449-19.10.2829130.0000200.0007360.0000140.019060.000537.3627
Kuma-449-20.10.2828970.0000250.0007530.0000070.020420.000306.7660
Kuma-449-21.10.2828570.0000210.0001690.0000050.004580.000175.4736
Kuma-449-22.10.2829100.0000200.0007750.0000060.020430.000287.3633
Kuma-449-23.10.2829020.0000240.0014360.0000210.038380.000427.0651
Kuma-449-24.10.2829180.0000260.0009340.0000330.026360.000837.5618
Kuma-449-25.10.2829030.0000210.0008090.0000110.021310.000206.9648
Kuma-449-26.10.2829080.0000200.0008300.0000110.025210.000237.2637
Kuma-449-27.10.2829260.0000240.0016100.0000210.043510.000157.7605
Kuma-449-28.10.2829180.0000200.0008420.0000040.021910.000317.5617
Kuma-449-29.10.2829060.0000270.0006180.0000040.016170.000307.2638
Kuma-449-29.20.2829310.0000220.0007170.0000160.021560.000658.0590
Kuma-449-30.10.2829470.0000210.0007210.0000060.018150.000308.5560
Kuma-450
Kuma-450-1.10.2829280.0000240.0015190.0000110.042620.000737.9599
Kuma-450-1.20.2829130.0000230.0007870.0000210.021780.000537.4626
Kuma-450-2.10.2829030.0000250.0014220.0000340.041000.001307.0649
Kuma-450-3.10.2824870.0000280.0009040.0000280.026060.00030−7.81469
Kuma-450-4.10.2829300.0000330.0028220.0000200.083400.001607.8601
Kuma-450-5.10.2828880.0000270.0016720.0000420.049300.000316.4680
Kuma-450-6.10.2829260.0000240.0012520.0000270.033940.000697.8602
Kuma-450-7.10.2828790.0000220.0010850.0000120.031560.000366.2695
Kuma-450-8.10.2828990.0000280.0016350.0000270.046700.001406.8658
Kuma-450-9.10.2829170.0000280.0016980.0000610.043900.001407.5622
Kuma-450-10.10.2829330.0000270.0019560.0000140.056540.000447.9593
Kuma-450-11.10.2829110.0000300.0027690.0000200.080770.000897.1640
Kuma-450-12.10.2829200.0000260.0011870.0000190.031740.000257.6615
Kuma-450-13.10.2829270.0000220.0006520.0000100.019420.000507.8600
Kuma-450-14.10.2829230.0000220.0008720.0000010.025470.000287.7608
Kuma-5
Kuma-5-1.10.2814360.0000240.0006980.0000170.021890.00065−1.72697
Kuma-5-1.20.2814400.0000220.0006490.0000120.020750.00043−0.82673
Kuma-5-2.10.2827240.0000270.0011430.0000250.034550.000510.11012
Kuma-5-3.10.2815560.0000260.0009960.0000330.025160.000583.42467
Kuma-5-4.10.2827950.0000230.0012170.0000290.037300.001002.8868
Kuma-5-5.10.2815830.0000210.0006970.0000400.022700.00120−1.02498
Kuma-5-6.10.2814400.0000190.0005530.0000080.015060.000241.62624
Kuma-5-7.10.2827970.0000200.0006110.0000060.018120.000213.0862
Kuma-5-8.10.2815780.0000210.0011370.0000130.036430.00078−1.82539
Kuma-5-9.10.2816420.0000280.0013680.0000540.044800.00260−0.22438
Kuma-5-10.10.2814100.0000220.0007400.0000100.023300.00038−0.42708
Kuma-5-11.10.2815150.0000190.0002900.0000250.009320.00079−3.32609
Kuma-5-12.10.2822880.0000250.0011090.0000110.033000.00046−15.11865
Kuma-5-13.10.2823020.0000520.0011200.0000120.030820.00040−14.71839
Kuma-5-14.10.2828390.0000400.0015600.0000390.049000.002104.2786
Kuma-5-15.10.2828670.0000370.0020310.0000360.061700.001605.1732
Kuma-5-16.10.2821880.0000260.0014020.0000180.044950.00062−18.72060
Kuma-5-17.10.2815580.0000190.0005710.0000310.017390.00087−1.12526
Kuma-5-18.10.2827530.0000220.0008100.0000080.023760.000434.8885
Kuma-5-18.20.2827620.0000190.0011160.0000060.031520.000244.9874
Kuma-5-19.10.2828060.0000350.0029020.0000790.087200.002102.9855
Kuma-5-20.10.2821190.0000180.0004060.0000060.012360.00018−19.62163
Kuma-5-21.10.2829360.0000270.0006900.0000090.018980.000308.2580
Kuma-5-22.10.2816610.0000210.0007820.0000040.024350.000321.52357
Kuma-5-23.10.2827580.0000250.0011570.0000090.030000.000472.0932
Kuma-5-24.10.2827170.0000510.0013730.0000170.038140.000622.6977
Kuma-5-25.10.2821230.0000230.0018190.0000220.057500.00100−21.12189
Kuma-5-26.10.2814810.0000250.0012020.0000230.039300.001300.92620
Kuma-5-27.10.2813120.0000240.0004940.0000060.015270.000190.32805
Kuma-5-28.10.2815740.0000180.0006310.0000380.022100.00150−1.22510
Kuma-5-29.10.2828800.0000200.0003790.0000030.011410.000109.3632
Kuma-6
Kuma-6-1.10.2828580.0000280.0024200.0001100.077400.004105.4741
Kuma-6-2.10.2828060.0000270.0016890.0000130.049670.000573.6842
Kuma-6-3.10.2828260.0000260.0012150.0000200.037300.001204.3800
Kuma-6-4.10.2828550.0000290.0016300.0000530.045000.002005.3744
Kuma-6-5.10.2828070.0000220.0011640.0000180.035160.000633.7836
Kuma-6-6.10.2828560.0000300.0016050.0000090.047250.000685.4741
Kuma-6-7.10.2828760.0001100.0016410.0000760.062200.001606.0703
Kuma-6-8.10.2828530.0000340.0012120.0000100.036560.000795.3746
Kuma-6-9.10.2828300.0000270.0018300.0000210.055620.000404.5794
Kuma-6-10.10.2828710.0000280.0019940.0000680.058800.002105.9714
Kuma-6-11.10.2828310.0000300.0021760.0000530.069600.001704.3795
Kuma-6-12.10.2828240.0000230.0014260.0000120.042040.000644.3803
Table A3. LA-MC-ICPMS Lu-Yb-Hf isotopic compositions of the detrital zircons from the Hayang Group, Korea.
Table A3. LA-MC-ICPMS Lu-Yb-Hf isotopic compositions of the detrital zircons from the Hayang Group, Korea.
Spot No.176Hf/177Hf±2 s.d.176Lu/177Hf±2 s.d.176Yb/177Hf±2 s.d.Apparent Age (Ma)εHf(t)T2DM (Ma)
Chilgok Formation
ChG-1_1.10.2824620.0000340.0007770.0000320.0236500.000440114.2−8.51515
ChG-1_2.10.2823630.0000210.0006030.0000100.0212500.000500111.5−12.11709
ChG-1_3.10.2824050.0000230.0005520.0000150.0162800.000230110.0−10.61628
ChG-1_4.10.2822810.0000240.0011850.0000130.0408400.000470107.9−15.11873
ChG-1_5.10.2821590.0000130.0001350.0000060.0052600.000220158.9−18.22085
ChG-1_6.10.2824020.0000360.0010100.0000350.0322000.001100108.9−10.81636
ChG-1_7.10.2822860.0000330.0009750.0000320.0310500.000780111.7−14.81861
ChG-1_8.10.2812900.0000270.0002920.0000040.0107400.0001901958.0−9.22998
ChG-1_9.10.2822600.0000190.0007550.0000140.0265600.000510108.3−15.81912
ChG-1_10.10.2822510.0000190.0005990.0000190.0182500.000220108.2−16.11929
ChG-1_11.10.2823100.0000190.0005030.0000120.0174900.000470111.5−13.91813
ChG-1_12.10.2823060.0000230.0009530.0000450.0258800.000780109.6−14.11823
ChG-1_13.10.2823870.0000230.0007240.0000480.0237000.001700109.5−11.31664
ChG-1_14.10.2810480.0000180.0003290.0000030.0100200.0001102373.0−8.43285
ChG-1_15.10.2822450.0000220.0004720.0000080.0166800.000300110.1−16.31940
ChG-1_16.10.2823470.0000200.0006200.0000100.0193100.000420107.8−12.71742
ChG-1_17.10.2814220.0000250.0009140.0000120.0319200.000310817.4−30.33247
ChG-1_18.10.2823290.0000260.0011500.0001100.0364000.002500109.1−13.41779
ChG-1_19.10.2813300.0000210.0005710.0000260.0167700.0002701682.0−14.33056
ChG-1_20.10.2823130.0000260.0010280.0000430.0395000.001500108.5−13.91810
ChG-1_21.10.2807500.0000170.0004720.0000100.0160700.0002202728.0−11.23712
ChG-1_22.10.2811250.0000180.0005150.0000100.0169600.0003902162.0−10.73243
ChG-1_23.10.2821720.0000180.0004190.0000050.0134800.000140185.4−17.22051
ChG-1_24.10.2821860.0000190.0006290.0000060.0212000.000320165.9−17.22033
ChG-1_25.10.2821900.0000160.0005970.0000070.0191100.000350164.3−17.02025
ChG-1_26.10.2823190.0000190.0004360.0000030.0159900.000150110.2−13.61795
ChG-1_27.10.2822800.0000170.0002360.0000030.0080100.000110816.60.51571
ChG-1_28.10.2822980.0000270.0008380.0000270.0290600.000820109.5−14.41838
ChG-1_29.10.2824520.0000520.0015040.0000710.0377000.001600108.9−9.01539
ChG-1_30.10.2815210.0000220.0006330.0000330.0252000.0012001273.0−16.62862
ChG-1_31.10.2824050.0000180.0002230.0000040.0081430.000095106.7−10.71628
ChG-1_32.10.2822730.0000190.0005980.0000140.0186200.000240108.4−15.31886
ChG-1_33.10.2821770.0000160.0001260.0000040.0048200.000120163.1−17.52049
ChG-1_34.10.2812700.0000170.0002910.0000040.0107300.0001201782.0−13.83111
ChG-1_35.10.2813450.0000220.0006870.0000230.0256000.0010001659.0−14.43044
ChG-1_36.10.2822720.0000200.0004500.0000040.0161400.000170106.9−15.41889
ChG-1_37.10.2822850.0000200.0005640.0000040.0196600.000210104.5−15.01865
ChG-1_38.10.2822790.0000260.0007060.0000050.0253500.000120109.9−15.11875
ChG-1_39.10.2822930.0000200.0005100.0000070.0178400.000270107.6−14.61847
Silla Conglomerate
Sila14_1.10.2816770.0000300.0017280.0000410.0473900.0006201833.70.02406
Sila14_2.10.2820440.0000220.0004010.0000050.0106000.000200165.0−22.22308
Sila14_3.10.2815290.0000200.0003130.0000100.0087400.0003001848.1−3.22590
Sila14_4.10.2825350.0000340.0014510.0000350.0351800.000830835.09.31101
Sila14_5.10.2822580.0000220.0005700.0000060.0148600.000150174.4−14.41888
Sila14_6.10.2821770.0000340.0015130.0000240.0447000.001200780.8−4.61823
Sila14_7.10.2822800.0000230.0007930.0000060.0199000.000300111.3−15.01872
Sila14_8.10.2816700.0000200.0003550.0000020.0097750.0000801841.71.62325
Sila14_9.10.2805920.0000270.0008840.0000060.0238100.0001402042.7−32.94323
Sila14_10.10.2820730.0000240.0003980.0000060.0098100.000210164.3−21.22252
Sila14_11.10.2824380.0000290.0004940.0000050.0106600.000200798.45.51277
Sila14_12.10.2817480.0000280.0002600.0000040.0070000.0002001304.9−7.52396
Sila14_13.10.2821000.0000320.0013770.0000300.0363000.001400789.6−7.11965
Sila14_14.10.2813300.0000210.0003190.0000050.0095900.0001701038.3−28.33312
Sila14_15.10.2821260.0000250.0006920.0000320.0163900.000630163.6−19.32151
Sila14_16.10.2822920.0000290.0015160.0000390.0409200.000750113.9−14.61850
Sila14_17.10.2805950.0000270.0002830.0000000.0080690.0000782539.6−20.64064
Sila14_18.10.2820440.0000220.0005410.0000010.0159100.0001401217.50.81873
Sila14_19.10.2823000.0000220.0003310.0000030.0080700.000110823.41.31532
Sila14_20.10.2825150.0000510.0010890.0000500.0264800.000880107.2−6.81415
Sila14_21.10.2824550.0000710.0007590.0000060.0215500.0001501352.718.21027
Sila14_22.10.2821620.0000250.0005810.0000110.0140500.000250114.4−19.12100
Sila14_23.10.2824740.0000160.0002670.0000080.0067100.000210237.9−5.41437
KU5_1.10.2822510.0000220.0004900.0000110.0116000.000250181.9−14.51898
KU5_2.10.2817860.0000220.0007280.0000360.0188000.0010001919.07.02095
KU5_3.10.2816790.0000290.0005000.0000020.0129360.0000841879.02.62302
KU5_4.10.2813810.0000180.0007550.0000120.0175500.0002602177.0−1.72769
KU5_5.10.2821380.0000210.0006020.0000080.0132000.0002801159.02.81717
KU5_6.10.2820490.0000190.0006830.0000060.0156660.000085394.3−17.12206
KU5_7.10.2824840.0000240.0014820.0000140.0342300.000270228.2−5.41431
KU5_8.10.2819040.0000230.0014960.0000150.0372700.000510760.1−14.72359
KU5_9.10.2814190.0000240.0003600.0000060.0090600.0001302091.0−1.72701
KU5_10.10.2813450.0000290.0001750.0000170.0044800.0003802067.0−4.62839
KU5_11.10.2822370.0000230.0004730.0000210.0112100.000480172.2−15.21930
KU5_12.10.2820790.0000180.0004330.0000040.0100500.000091166.5−20.92239
KU5_13.10.2813790.0000250.0007480.0000130.0170100.0002602527.06.22630
KU5_14.10.2820300.0000210.0006020.0000070.0142100.000180184.9−22.32328
KU5_15.10.2818830.0000260.0005100.0000070.0137700.0002701208.0−5.12188
KU5_16.10.2821770.0000340.0004210.0000070.0090200.000140186.4−17.02040
KU5_17.10.2820660.0000180.0003110.0000040.0068370.000062165.4−21.42264
KU5_18.10.2816110.0000240.0004190.0000070.0106900.0002001883.00.42425
KU5_19.10.2812670.0000240.0002380.0000020.0061260.0000452398.00.12851
KU5_20.10.2823230.0000190.0002270.0000320.0058000.000780385.2−7.51670
KU5_21.10.2824770.0000280.0007000.0000230.0175700.000550178.3−6.61459
KU5_22.10.2821370.0000340.0016060.0000660.0403000.001900119.1−20.02151
KU5_23.10.2820890.0000350.0007600.0000200.0173100.000580111.4−21.82244
KU5_24.10.2812950.0000200.0003810.0000030.0092940.0000532376.00.42820
KU5_25.10.2822640.0000200.0008470.0000150.0201700.000370108.4−15.71905
KU5_26.10.2819500.0000250.0004660.0000050.0126200.0002001014.4−7.02137
KU5_27.10.2814510.0000180.0002730.0000150.0069100.0003701919.0−4.32706
KU5_28.10.2821630.0000270.0004650.0000040.0122300.0001301152.03.61666
KU5_29.10.2820880.0000190.0000790.0000030.0022750.000085882.5−4.81912
KU5_30.10.2823080.0000190.0005020.0000100.0119000.000180104.8−14.11819
KU5_31.20.2821600.0000180.0004330.0000100.0100200.000280182.5−17.72075
KU5_33.10.2821730.0000300.0007380.0000250.0189900.000710181.5−17.32052
KU5_34.10.2821570.0000160.0003790.0000030.0079900.000093168.9−18.12086
KU5_35.10.2822960.0000220.0010850.0000030.0259300.000059191.5−12.81811
KU5_37.10.2821080.0000260.0005100.0000060.0119400.000150109.6−21.12207
KU5_38.10.2812880.0000210.0003220.0000030.0075040.0000692582.04.92741
KU5_39.10.2821110.0000210.0007180.0000080.0176700.000160392.0−15.02087
KU5_40.10.2821800.0000240.0005360.0000090.0126900.000170169.6−17.32042
KU5_41.10.2822130.0000210.0005100.0000090.0114300.000160109.7−17.42003
Haman Formation.
HA-1_1.10.2821170.0000330.0003410.0000170.0084500.000420110.3−20.82189
HA-1_2.10.2822950.0000210.0005190.0000130.0132600.000390111.5−14.51842
HA-1_3.10.2822890.0000180.0004430.0000020.0114140.000072110.2−14.71854
HA-1_4.10.2823130.0000220.0009340.0000190.0227400.000450109.2−13.91809
HA-1_5.10.2815590.0000190.0002670.0000130.0075500.0003301865.9−1.72522
HA-1_6.10.2821140.0000300.0005750.0000160.0139900.000270114.7−20.82193
HA-1_7.10.2822320.0000310.0011610.0000510.0286000.001300113.9−16.71966
HA-1_8.10.2821590.0000270.0005600.0000140.0124300.000230116.2−19.22105
HA-1_9.10.2821180.0000270.0011700.0000070.0280800.000310116.1−20.72187
HA-1_10.10.2821560.0000280.0008540.0000090.0213200.000500116.4−19.32112
HA-1_11.10.2822990.0000230.0006850.0000080.0175100.000100174.0−13.01809
HA-1_12.10.2823090.0000350.0009490.0000110.0257300.000150172.4−12.71792
HA-1_13.10.2821390.0000220.0006400.0000050.0163400.000330115.6−19.92145
HA-1_14.10.2821220.0000240.0007540.0000280.0177900.000540117.4−20.52177
HA-1_15.10.2821110.0000240.0008930.0000260.0226200.000410114.9−20.92200
HA-1_16.10.2822690.0000280.0007780.0000150.0202800.000420113.0−15.41893
HA-1_17.10.2823250.0000210.0005470.0000040.0148270.000086111.4−13.41783
HA-1_18.10.2822500.0000190.0005300.0000060.0126800.000220114.3−16.01929
HA-1_19.10.2821890.0000200.0007100.0000050.0168500.000160112.3−18.22049
HA-1_20.10.2823120.0000180.0004980.0000110.0130300.000370114.3−13.81808
HA-1_21.10.2822970.0000210.0007660.0000080.0203800.000140111.6−14.41839
HA-1_22.10.2820470.0000240.0008120.0000050.0201400.000210115.7−23.22324
HA-1_23.10.2822170.0000250.0007210.0000080.0185400.000360111.6−17.21995
HA-1_24.10.2821450.0000210.0007220.0000100.0173000.000240113.8−19.72134
HA-1_25.10.2823250.0000200.0005280.0000040.0132390.000074109.1−13.51784
HA-1_26.10.2821460.0000190.0004570.0000040.0122900.000110113.5−19.72131
HA-1_27.10.2822330.0000190.0004400.0000080.0106700.000240114.0−16.61962
HA-1_28.10.2820660.0000170.0001240.0000090.0032300.000250118.0−22.42284
HA-1_29.10.2823090.0000200.0007030.0000100.0188200.000280171.2−12.71791
HA-1_30.10.2822080.0000190.0007340.0000110.0173200.000240112.4−17.52012
HA-1_31.10.2814630.0000190.0005880.0000170.0162800.0004801973.8−3.12683
HA-1_32.10.2823240.0000280.0007660.0000080.0203700.000220111.9−13.51786
HA-1_33.10.2824620.0000220.0006020.0000070.0168300.000310223.0−6.21470
HA-1_34.10.2821710.0000290.0009050.0000210.0225100.000350116.7−18.82083
HA-1_35.10.2821450.0000320.0010170.0000210.0236300.000460113.6−19.82135
HA-1_36.10.2815230.0000180.0009120.0000050.0239300.000120761.7−27.93076
HA-1_37.10.2822840.0000190.0004680.0000050.0122700.000200109.7−14.91864
HA-1_38.10.2824110.0000150.0002560.0000020.0061000.000110264.9−7.01549
HA-1_39.10.2814990.0000180.0009050.0000060.0258000.0001501865.4−4.62680
HA-1_40.10.2820530.0000370.0005610.0000090.0150500.000280116.1−22.92311
HA-1_41.10.2821750.0000200.0006930.0000190.0180100.000590113.2−18.72076
HA-1_42.10.2822510.0000230.0007360.0000580.0201000.001500108.3−16.11930
HA-1_43.10.2821010.0000200.0006700.0000130.0166800.000360115.7−21.22219
HA-1_44.10.2814490.0000170.0011840.0000120.0341500.0003801849.4−7.12801
HA-1_45.10.2822480.0000240.0007970.0000090.0195700.000190116.9−16.01932
HA-1_46.10.2821180.0000230.0004990.0000060.0132200.000260103.5−20.92190
HA-1_47.10.2821740.0000360.0008870.0000410.0212200.000830114.6−18.72078
HA-1_48.10.2823530.0000200.0006740.0000050.0170000.000170110.4−12.41730
HA-1_49.10.2814290.0000180.0007270.0000530.0191000.0014001271.0−20.03043
HA-1_50.10.2822340.0000230.0012700.0000310.0334200.000610112.7−16.71963
HA-1_51.10.2822890.0000190.0005600.0000060.0146800.000190110.6−14.71854
HA-1_52.10.2822980.0000190.0005610.0000050.0145700.000170110.2−14.41837
HA-1_53.10.2822460.0000170.0004100.0000060.0113700.000210189.2−14.51905
HA-1_54.10.2821880.0000180.0006700.0000140.0152000.000250187.5−16.62020
HA-1_55.10.2821280.0000220.0009770.0000060.0246600.000100107.3−20.52171
HA-1_56.10.2824270.0000190.0004880.0000080.0135800.000330217.0−7.51540
HA-1_57.10.2811950.0000170.0006390.0000020.0171850.0000901906.8−14.13224
HA-1_58.10.2814170.0000160.0002010.0000030.0053260.0000662459.06.92536
HA-1_59.10.2822630.0000210.0007440.0000100.0203900.000200437.1−8.61773
HA-1_60.10.2821540.0000270.0007920.0000090.0188300.000200114.2−19.42117
HA-1_61.10.2811150.0000190.0005360.0000020.0144300.0001101914.0−16.73366
HA-1_62.10.2823480.0000220.0005400.0000090.0149900.000220222.1−10.21693
HA-1_63.10.2824200.0000190.0006280.0000070.0175300.000140223.6−7.61552
HA-1_64.10.2814940.0000150.0001590.0000090.0046800.0002201635.9−9.02737
HA-1_65.10.2822030.0000280.0007230.0000340.0177200.000970184.8−16.21992
HA-1_66.10.2820530.0000170.0004380.0000070.0112200.000220113.3−23.02312
HA-1_67.10.2821200.0000210.0007370.0000100.0175700.000130106.9−20.82186
HA-1_68.10.2821600.0000210.0007170.0000130.0177700.000410114.2−19.22105
HA-1_69.10.2822540.0000250.0006510.0000140.0188600.000530216.9−13.71879
HA-1_70.10.2823150.0000190.0005140.0000040.0137300.000220110.2−13.81803
Jindong Formation
JD-2-1_1.10.2829310.0000300.0010830.0000430.0247800.000780103.07.8595
JD-2-1_2.10.2828200.0000280.0007870.0000150.0203500.000260108.84.0812
JD-2-1_3.10.2829610.0000170.0007420.0000060.0171900.000080270.312.5467
JD-2-1_4.10.2825360.0000330.0011960.0000080.0313900.00047099.1−6.31377
JD-2-1_5.10.2827820.0000260.0011490.0000310.0295000.000500108.32.6889
JD-2-1_6.10.2828070.0000260.0007140.0000180.0190300.000320105.63.5839
JD-2-1_7.10.2828010.0000280.0009210.0000490.0220700.000900102.83.2852
JD-2-1_8.10.2827800.0000250.0013210.0000420.0340000.001000102.82.4895
JD-2-1_9.10.2829430.0000200.0007620.0000190.0194800.000520270.611.9502
JD-2-1_10.10.2829130.0000190.0005650.0000040.0135500.000210277.911.0557
JD-2-1_11.10.2829510.0000300.0008780.0000140.0222300.000420104.28.6554
JD-2-1_12.10.2829630.0000350.0016560.0000270.0435900.000640273.012.5471
JD-2-1_13.10.2829720.0000470.0014130.0000460.0343000.001500103.79.3515
JD-2-1_14.10.2829520.0000260.0006780.0000100.0169800.000250271.412.2483
JD-2-1_15.10.2829200.0000240.0004090.0000120.0086600.000210294.511.6535
JD-2-1_16.10.2828880.0000300.0014090.0000070.0388200.000200107.36.4680
JD-2-1_17.10.2825450.0000320.0010140.0000300.0275300.000500100.3−5.91358
JD-2-1_18.10.2828780.0000230.0009390.0000170.0222400.000240102.05.9700
JD-2-1_19.10.2829810.0000280.0010830.0000340.0292000.001200271.613.2430
JD-2-1_20.10.2819440.0000300.0010010.0000160.0267300.000280109.2−27.02526
JD-2-1_21.10.2829320.0000190.0004650.0000020.0120330.000085264.711.4524
JD-2-1_22.10.2829760.0000360.0011700.0000300.0275000.001000283.513.2436
JD-2-1_23.10.2825000.0000260.0010490.0000160.0282200.00043098.8−7.51448
JD-2-1_24.10.2829420.0000230.0011110.0000120.0273300.000150300.012.4496
JD-2-1_25.10.2829330.0000240.0010770.0000150.0271500.000350275.811.6523
JD-2-1_26.10.2829010.0000150.0005670.0000290.0129200.000500234.29.6599
JD-2-1_27.10.2825320.0000280.0011060.0000340.0277000.00066098.5−6.41385
JD-2-1_28.10.2829910.0000380.0018220.0000090.0432300.000210290.013.8411

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Figure 1. Geological map of the Gyeongsang basin in southeastern Korea (after Lee et al. 2018) [19] and the Amakusa Islands (after Saito et al. 2010) [23] with sample locations. (a) East Asia map including Korea and Japan. The positions of Kyushu and the Gyeongsang Basin are marked in red. (b) The inset within Kyushu marks the location of the Amakusa Islands and Uto Peninsula, where the Cretaceous Himenoura and Goshoura groups are distributed. (c) The distribution of the Cretaceous Himenoura and Goshoura groups and sampling locations from them are shown. (d) It is a schematic geological map of the Cretaceous Gyeongsang basin and also shows the sampling locations in the Hayang Group.
Figure 1. Geological map of the Gyeongsang basin in southeastern Korea (after Lee et al. 2018) [19] and the Amakusa Islands (after Saito et al. 2010) [23] with sample locations. (a) East Asia map including Korea and Japan. The positions of Kyushu and the Gyeongsang Basin are marked in red. (b) The inset within Kyushu marks the location of the Amakusa Islands and Uto Peninsula, where the Cretaceous Himenoura and Goshoura groups are distributed. (c) The distribution of the Cretaceous Himenoura and Goshoura groups and sampling locations from them are shown. (d) It is a schematic geological map of the Cretaceous Gyeongsang basin and also shows the sampling locations in the Hayang Group.
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Figure 2. Cathodoluminescence images of studied zircons from the Goshoura and Himenoura Groups. The red and blue ellipses represent U-Pb analysis and Hf analysis spots, respectively. Four samples are shown separately; (a) Kuma-449, (b) Kuma-450, (c) Kuma-5, and (d) Kuma-6. The size of spots for Hf isotope analysis (blue) is larger than spots in U-Pb analysis (red). Only the zircon grains of Kuma-5 contain ages older than Cretaceous and those with more developed roundness than other samples.
Figure 2. Cathodoluminescence images of studied zircons from the Goshoura and Himenoura Groups. The red and blue ellipses represent U-Pb analysis and Hf analysis spots, respectively. Four samples are shown separately; (a) Kuma-449, (b) Kuma-450, (c) Kuma-5, and (d) Kuma-6. The size of spots for Hf isotope analysis (blue) is larger than spots in U-Pb analysis (red). Only the zircon grains of Kuma-5 contain ages older than Cretaceous and those with more developed roundness than other samples.
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Figure 3. Tera-Wasserburg diagrams of SHRIMP U-Pb detrital zircon ages from the (a,b) Goshoura Group and (c,d) Himenoura Group.
Figure 3. Tera-Wasserburg diagrams of SHRIMP U-Pb detrital zircon ages from the (a,b) Goshoura Group and (c,d) Himenoura Group.
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Figure 4. Cathodoluminescence images of studied zircons from the Hayang Group. The small ellipses are the spots for the previous U-Pb age analysis, and the large ellipses are the spots for the Hf analysis.
Figure 4. Cathodoluminescence images of studied zircons from the Hayang Group. The small ellipses are the spots for the previous U-Pb age analysis, and the large ellipses are the spots for the Hf analysis.
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Figure 5. Plot of zircon εHf(t) versus crystallization ages. The evolutionary path of the depleted mantle is based on 176Lu/177Hf and 176Hf/177Hf ratios from Griffin et al. [48]. The evolution lines for the continental crust with ages of 2500 Ma and 3500 Ma were drawn using the Lu/Hf ratio (=0.081) of Rudnick and Gao [49]. (a) Plot of zircon εHf(t) versus crystallization ages for the entire age range. (b) A plot expanded only in the range of about 80–300 Ma.
Figure 5. Plot of zircon εHf(t) versus crystallization ages. The evolutionary path of the depleted mantle is based on 176Lu/177Hf and 176Hf/177Hf ratios from Griffin et al. [48]. The evolution lines for the continental crust with ages of 2500 Ma and 3500 Ma were drawn using the Lu/Hf ratio (=0.081) of Rudnick and Gao [49]. (a) Plot of zircon εHf(t) versus crystallization ages for the entire age range. (b) A plot expanded only in the range of about 80–300 Ma.
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Lee, T.-H.; Park, K.-H. Detrital Zircon U-Pb Geochronology and Hf Isotope Geochemistry of the Hayang Group, SE Korea and the Himenoura and Goshoura Groups, SW Japan: Signs of Subduction-Related Magmatism after a Long Resting Period. Minerals 2020, 10, 936. https://doi.org/10.3390/min10110936

AMA Style

Lee T-H, Park K-H. Detrital Zircon U-Pb Geochronology and Hf Isotope Geochemistry of the Hayang Group, SE Korea and the Himenoura and Goshoura Groups, SW Japan: Signs of Subduction-Related Magmatism after a Long Resting Period. Minerals. 2020; 10(11):936. https://doi.org/10.3390/min10110936

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Lee, Tae-Ho, and Kye-Hun Park. 2020. "Detrital Zircon U-Pb Geochronology and Hf Isotope Geochemistry of the Hayang Group, SE Korea and the Himenoura and Goshoura Groups, SW Japan: Signs of Subduction-Related Magmatism after a Long Resting Period" Minerals 10, no. 11: 936. https://doi.org/10.3390/min10110936

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