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Article
Peer-Review Record

Preparation of Alkaline Polyelectrolyte Membrane Based on Quaternary Ammonium Salt–Modified Cellulose and Its Application in Zn–Air Flexible Battery

Polymers 2021, 13(1), 9; https://doi.org/10.3390/polym13010009
by Xiang You 1,2,†, Congde Qiao 1,2,†, Dan Peng 3, Weiliang Liu 1,2, Cong Li 4, Hui Zhao 1,2,5, Hao Qi 1,2, Xiaoxia Cai 1,2,*, Yanqiu Shao 3,* and Xinhua Shi 3
Reviewer 1: Anonymous
Reviewer 2: Anonymous
Polymers 2021, 13(1), 9; https://doi.org/10.3390/polym13010009
Submission received: 19 November 2020 / Revised: 16 December 2020 / Accepted: 18 December 2020 / Published: 22 December 2020
(This article belongs to the Special Issue Polymer Materials for Electrochemical Applications)

Round 1

Reviewer 1 Report

The manuscript "Preparation of alkaline polyelectrolyte membrane  based on quaternary ammonium salt modified cellulose and its application in Zn-Air flexible battery"  describes a new method of preparation of alkaline polyelectrolyte membrane. The research may be of interest for the readers of the "Polymers" journal, however, some points need to be clarified.

1) Lines 176-188 Please, specify exact amounts of the components, used for preparation of electrodes slurry. 

2) Please, provide the manufacturer and model of the LED used for Zn-air battery test.

3) Provide some precise data on Zn-air battery (EMF, power/current and volt/ampere characteristics)

Minor points:

Line 43 - replace "polymer solid electrolyte (SPE)" with "solid polymer electrolyte (SPE)"

Line 113 - please, correct the typos in the frequency values - superscript is missing.

Line 121 -  at 10 mV s-1 superscript is missing

Author Response

Please see the attachment

Author Response File: Author Response.docx

Reviewer 2 Report

The manuscript compares polymer electrolytes with different mechanical supports, MCC, and QMCC. Although their results show the improvements in mechanical properties, condcutivities. I can't see any insights from the manuscript and the discussions are too general. I think the manuscript is not suitable for publication. My other comments:

  1. The FTIR is not convincing as evidence for the success of grafting, the curves are two close, do they have other evidence? 
  2. Why the authors label the sample with loading (e.g.4g), not weight fraction?
  3. The comparison of the Zn-air battery should be quantified, not by simple demonstration, therefore the electrochemical performance tests performances are necessary. 

Author Response

Please see the attachment

Author Response File: Author Response.docx

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